Intercalation Pseudocapacitance in 2D VS2/Ti3C2Tx MXene Hybrids for All‐Climate and Long‐Cycle Sodium‐Ion Batteries Article Swipe
Zhenyun Zhao
,
Yang Wu
,
Rui Hu
,
Jianguo Lü
,
Dongliang Chen
,
Tongtong Li
,
Yunna Guo
,
Liqiang Zhang
,
Hongwen Chen
,
Zhizhen Ye
,
Chuanfang Zhang
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202307794
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202307794
Layered transition metal dichalcogenides have great potential as anodes of sodium‐ion batteries (SIBs) due to their high theoretical specific capacity. However, the restacking severely limits their accessible sites, leading to undesirable specific capacity, cycle stability, and working temperature range. Herein, a hierarchical 2D VS 2 /Ti 3 C 2 T x MXene hybrid is designed via a simple liquid‐mixing method, where VS 2 is confined in the conductive Ti 3 C 2 T x matrix with chemical connections built between them. The in situ transmission electron microscopy analyses reveal that the hybrid depends on a very fast and reversible intercalation/de‐intercalation process between VS 2 and Na x VS 2 (where x = 1) to store sodium. Theoretical calculations disclose that the Ti 3 C 2 T x matrix remarkably enhances the charge transfer and alleviates the volume expansion of VS 2 especially after Na + is inserted. Consequently, such a rational design exhibits an intercalation pseudocapacitance‐dominant mechanism, with excellent specific capacity (522 mAh g −1 at 0.2 A g −1 ), rate capability (342 mAh g −1 at 10 A g −1 ), cycle life (116% after 3000 cycles), and also all‐climate workability (with high specific capacity and long‐term cycle stability even at 70 and −40 °C). This study may open up a new vision to design fast‐charging, long‐cycle, and all‐climate SIBs anodes based on the intercalation pseudocapacitance.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adfm.202307794
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202307794
- OA Status
- bronze
- Cited By
- 54
- References
- 42
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4386481858
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4386481858Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adfm.202307794Digital Object Identifier
- Title
-
Intercalation Pseudocapacitance in 2D VS2/Ti3C2Tx MXene Hybrids for All‐Climate and Long‐Cycle Sodium‐Ion BatteriesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-09-05Full publication date if available
- Authors
-
Zhenyun Zhao, Yang Wu, Rui Hu, Jianguo Lü, Dongliang Chen, Tongtong Li, Yunna Guo, Liqiang Zhang, Hongwen Chen, Zhizhen Ye, Chuanfang ZhangList of authors in order
- Landing page
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https://doi.org/10.1002/adfm.202307794Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202307794Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
bronzeOpen access status per OpenAlex
- OA URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202307794Direct OA link when available
- Concepts
-
Pseudocapacitance, Intercalation (chemistry), Materials science, Ion, Chemical engineering, Sodium, Nanotechnology, Inorganic chemistry, Metallurgy, Electrochemistry, Physical chemistry, Supercapacitor, Chemistry, Engineering, Electrode, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
54Total citation count in OpenAlex
- Citations by year (recent)
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2025: 34, 2024: 18, 2023: 2Per-year citation counts (last 5 years)
- References (count)
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42Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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