Interdependence of Support Wettability ‐ Electrodeposition Rate‐ Sodium Metal Anode and SEI Microstructure Article Swipe
Chang‐An Lo
,
Yixian Wang
,
Varun R. Kankanallu
,
Aditya Singla
,
Dean Yen
,
Xiaoyin Zheng
,
Kaustubh G. Naik
,
Bairav S. Vishnugopi
,
Callum J. Campbell
,
Vikalp Raj
,
Chonghang Zhao
,
Lu Ma
,
Jianming Bai
,
Feipeng Yang
,
Ruipeng Li
,
Mingyuan Ge
,
John Watt
,
Partha P. Mukherjee
,
David Mitlin
,
Yu-chen Karen Chen-Wiegart
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202412550
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202412550
This study examines how current collector support chemistry (sodiophilic intermetallic Na 2 Te vs. sodiophobic baseline Cu) and electrodeposition rate affect microstructure of sodium metal and its solid electrolyte interphase (SEI). Capacity and current (6 mAh cm −2 , 0.5–3 mA cm −2 ) representative of commercially relevant mass loading in anode‐free sodium metal battery (AF‐SMBs) are analyzed. Synchrotron X‐ray nanotomography and grazing‐incidence wide‐angle X‐ray scattering (GIWAXS) are combined with cryogenic ion beam (cryo‐FIB) microscopy. Highlighted are major differences in film morphology, internal porosity, and crystallographic preferred orientation e.g. (110) vs. (100) and (211) with support and deposition rate. Within the SEI, sodium fluoride (NaF) is more prevalent with Te−Cu versus sodium hydride (NaH) and sodium hydroxide (NaOH) with baseline Cu. Due to competitive grain growth the preferred orientation of sodium crystallites depends on film thickness. Mesoscale modeling delineates the role of SEI (ionic conductivity, morphology) on electrodeposit growth and onset of electrochemical instability.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/ange.202412550
- OA Status
- green
- Cited By
- 1
- References
- 79
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4403323783
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4403323783Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/ange.202412550Digital Object Identifier
- Title
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Interdependence of Support Wettability ‐ Electrodeposition Rate‐ Sodium Metal Anode and SEI MicrostructureWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-09-15Full publication date if available
- Authors
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Chang‐An Lo, Yixian Wang, Varun R. Kankanallu, Aditya Singla, Dean Yen, Xiaoyin Zheng, Kaustubh G. Naik, Bairav S. Vishnugopi, Callum J. Campbell, Vikalp Raj, Chonghang Zhao, Lu Ma, Jianming Bai, Feipeng Yang, Ruipeng Li, Mingyuan Ge, John Watt, Partha P. Mukherjee, David Mitlin, Yu-chen Karen Chen-WiegartList of authors in order
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https://doi.org/10.1002/ange.202412550Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/2477128Direct OA link when available
- Concepts
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Wetting, Anode, Microstructure, Metal, Materials science, Sodium, Chemical engineering, Metallurgy, Inorganic chemistry, Chemistry, Composite material, Electrode, Physical chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2025: 1Per-year citation counts (last 5 years)
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79Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.(211) | 94 |
| abstract_inverted_index.(NaF) | 105 |
| abstract_inverted_index.(NaH) | 114 |
| abstract_inverted_index.grain | 125 |
| abstract_inverted_index.major | 78 |
| abstract_inverted_index.metal | 25, 54 |
| abstract_inverted_index.onset | 151 |
| abstract_inverted_index.rate. | 99 |
| abstract_inverted_index.solid | 28 |
| abstract_inverted_index.study | 2 |
| abstract_inverted_index.(NaOH) | 118 |
| abstract_inverted_index.(SEI). | 31 |
| abstract_inverted_index.(ionic | 144 |
| abstract_inverted_index.Within | 100 |
| abstract_inverted_index.affect | 21 |
| abstract_inverted_index.growth | 126, 149 |
| abstract_inverted_index.sodium | 24, 53, 103, 112, 116, 131 |
| abstract_inverted_index.versus | 111 |
| abstract_inverted_index.0.5–3 | 40 |
| abstract_inverted_index.Te−Cu | 110 |
| abstract_inverted_index.X‐ray | 60, 65 |
| abstract_inverted_index.battery | 55 |
| abstract_inverted_index.current | 5, 34 |
| abstract_inverted_index.depends | 133 |
| abstract_inverted_index.hydride | 113 |
| abstract_inverted_index.loading | 50 |
| abstract_inverted_index.support | 7, 96 |
| abstract_inverted_index.(GIWAXS) | 67 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.Capacity | 32 |
| abstract_inverted_index.baseline | 16, 120 |
| abstract_inverted_index.combined | 69 |
| abstract_inverted_index.examines | 3 |
| abstract_inverted_index.fluoride | 104 |
| abstract_inverted_index.internal | 83 |
| abstract_inverted_index.modeling | 138 |
| abstract_inverted_index.relevant | 48 |
| abstract_inverted_index.Mesoscale | 137 |
| abstract_inverted_index.analyzed. | 58 |
| abstract_inverted_index.chemistry | 8 |
| abstract_inverted_index.collector | 6 |
| abstract_inverted_index.cryogenic | 71 |
| abstract_inverted_index.hydroxide | 117 |
| abstract_inverted_index.porosity, | 84 |
| abstract_inverted_index.preferred | 87, 128 |
| abstract_inverted_index.prevalent | 108 |
| abstract_inverted_index.delineates | 139 |
| abstract_inverted_index.deposition | 98 |
| abstract_inverted_index.interphase | 30 |
| abstract_inverted_index.scattering | 66 |
| abstract_inverted_index.thickness. | 136 |
| abstract_inverted_index.(AF‐SMBs) | 56 |
| abstract_inverted_index.Highlighted | 76 |
| abstract_inverted_index.Synchrotron | 59 |
| abstract_inverted_index.competitive | 124 |
| abstract_inverted_index.differences | 79 |
| abstract_inverted_index.electrolyte | 29 |
| abstract_inverted_index.microscopy. | 75 |
| abstract_inverted_index.morphology) | 146 |
| abstract_inverted_index.morphology, | 82 |
| abstract_inverted_index.orientation | 88, 129 |
| abstract_inverted_index.sodiophobic | 15 |
| abstract_inverted_index.(cryo‐FIB) | 74 |
| abstract_inverted_index.(sodiophilic | 9 |
| abstract_inverted_index.anode‐free | 52 |
| abstract_inverted_index.commercially | 47 |
| abstract_inverted_index.crystallites | 132 |
| abstract_inverted_index.instability. | 154 |
| abstract_inverted_index.wide‐angle | 64 |
| abstract_inverted_index.conductivity, | 145 |
| abstract_inverted_index.intermetallic | 10 |
| abstract_inverted_index.electrodeposit | 148 |
| abstract_inverted_index.microstructure | 22 |
| abstract_inverted_index.nanotomography | 61 |
| abstract_inverted_index.representative | 45 |
| abstract_inverted_index.electrochemical | 153 |
| abstract_inverted_index.crystallographic | 86 |
| abstract_inverted_index.electrodeposition | 19 |
| abstract_inverted_index.grazing‐incidence | 63 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 91 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 20 |
| citation_normalized_percentile.value | 0.59812361 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |