Intermixing‐Driven Surface and Bulk Ferromagnetism in the Quantum Anomalous Hall Candidate MnBi₆Te₁₀ Article Swipe

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A. Tcakaev , Bastian Rubrecht , Jorge I. Facio , V. B. Zabolotnyy , L. T. Corredor , Laura Folkers , Ekaterina Kochetkova , T. R. F. Peixoto , Philipp Kagerer , Simon Heinze , Hendrik Bentmann , Robert J. Green , Pierluigi Gargiani , Manuel Valvidares , E. Weschke , M. W. Haverkort , F. Reinert , Jeroen van den Brink , B. Büchner , A. U. B. Wolter , Anna Isaeva , V. Hinkov ·

YOU? · · 2023 · Open Access · · DOI: https://doi.org/10.1002/advs.202203239

The recent realizations of the quantum anomalous Hall effect (QAHE) in MnBi 2 Te 4 and MnBi 4 Te 7 benchmark the (MnBi 2 Te 4 )(Bi 2 Te 3 ) n family as a promising hotbed for further QAHE improvements. The family owes its potential to its ferromagnetically (FM) ordered MnBi 2 Te 4 septuple layers (SLs). However, the QAHE realization is complicated in MnBi 2 Te 4 and MnBi 4 Te 7 due to the substantial antiferromagnetic (AFM) coupling between the SLs. An FM state, advantageous for the QAHE, can be stabilized by interlacing the SLs with an increasing number n of Bi 2 Te 3 quintuple layers (QLs). However, the mechanisms driving the FM state and the number of necessary QLs are not understood, and the surface magnetism remains obscure. Here, robust FM properties in MnBi 6 Te 10 ( n = 2) with T c ≈ 12 K are demonstrated and their origin is established in the Mn/Bi intermixing phenomenon by a combined experimental and theoretical study. The measurements reveal a magnetically intact surface with a large magnetic moment, and with FM properties similar to the bulk. This investigation thus consolidates the MnBi 6 Te 10 system as perspective for the QAHE at elevated temperatures.

Related Topics

Ferromagnetism

Condensed Matter Physics

Concepts

Quantum anomalous Hall effect Ferromagnetism Antiferromagnetism Condensed matter physics Materials science Magnetism Topological insulator Magnetic moment Optoelectronics Quantum Hall effect Physics Magnetic field Quantum mechanics

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Type: article
Language: en
Landing Page: https://doi.org/10.1002/advs.202203239
PDF: https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202203239
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Cited By: 21
References: 99
Related Works: 10
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DOI: https://doi.org/10.1002/advs.202203239

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Title: Intermixing‐Driven Surface and Bulk Ferromagnetism in the Quantum Anomalous Hall Candidate MnBi₆Te₁₀

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Type: article

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Language: en

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Publication year: 2023

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Publication date: 2023-02-17

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Authors: A. Tcakaev, Bastian Rubrecht, Jorge I. Facio, V. B. Zabolotnyy, L. T. Corredor, Laura Folkers, Ekaterina Kochetkova, T. R. F. Peixoto, Philipp Kagerer, Simon Heinze, Hendrik Bentmann, Robert J. Green, Pierluigi Gargiani, Manuel Valvidares, E. Weschke, M. W. Haverkort, F. Reinert, Jeroen van den Brink, B. Büchner, A. U. B. Wolter, Anna Isaeva, V. Hinkov

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Landing page: https://doi.org/10.1002/advs.202203239

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Concepts: Quantum anomalous Hall effect, Ferromagnetism, Antiferromagnetism, Condensed matter physics, Materials science, Magnetism, Topological insulator, Magnetic moment, Optoelectronics, Quantum Hall effect, Physics, Magnetic field, Quantum mechanics

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Cited by: 21

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Intermixing‐Driven Surface and Bulk Ferromagnetism in the Quantum Anomalous Hall Candidate MnBi6Te10 Article Swipe

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Intermixing‐Driven Surface and Bulk Ferromagnetism in the Quantum Anomalous Hall Candidate MnBi₆Te₁₀ Article Swipe