Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 1: Observational data analysis Article Swipe
Xing Wei
,
Yanjie Shen
,
Xiao‐Ying Yu
,
Yang Gao
,
Huiwang Gao
,
Ming Chu
,
Yujiao Zhu
,
Xiaohong Yao
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.5194/acp-23-15325-2023
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.5194/acp-23-15325-2023
This study employed multiple techniques to investigate the contribution of grown new particles to the number concentration of cloud condensation nuclei (CCN) at various supersaturation (SS) levels at a rural mountain site in the North China Plain from 29 June to 14 July 2019. On 8 new particle formation (NPF) days, the total particle number concentrations (Ncn) were 8.4 ± 6.1×103 cm−3, which was substantially higher compared to 4.7 ± 2.6×103 cm−3 on non-NPF days. However, the CCN concentration (Nccn) at 0.2 % SS and 0.4 % SS on the NPF days was significantly lower than those observed on non-NPF days (p<0.05). This was due to the lower cloud activation efficiency of preexisting particles resulting from organic vapor condensation and smaller number concentrations of preexisting particles on NPF days. A case-by-case examination showed that the grown new particles only yielded a detectable contribution to Nccn at 0.4 % SS and 1.0 % SS during the NPF event on 1 July 2019, accounting for 12 % ± 11 % and 23 % ± 12 % of Nccn, respectively. The increased Nccn during two other NPF events and at 0.2 % SS on 1 July 2019 were detectable but determined mainly by varying preexisting particles rather than grown new particles. In addition, the hygroscopicity parameter values, concentrations of inorganic and organic particulate components, and surface chemical composition of different sized particles were analyzed in terms of chemical drivers to grow new particles. The results showed that the grown new particles via organic vapor condensation generally had no detectable contribution to Nccn but incidentally did. However, this conclusion was drawn from a small size of observational data, leaving more observations, particularly long-term observations and the growth of preexisting particles to the CCN required size, needed for further investigation.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.5194/acp-23-15325-2023
- OA Status
- gold
- Cited By
- 7
- References
- 144
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4389790902
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4389790902Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.5194/acp-23-15325-2023Digital Object Identifier
- Title
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Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 1: Observational data analysisWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
-
2023-12-15Full publication date if available
- Authors
-
Xing Wei, Yanjie Shen, Xiao‐Ying Yu, Yang Gao, Huiwang Gao, Ming Chu, Yujiao Zhu, Xiaohong YaoList of authors in order
- Landing page
-
https://doi.org/10.5194/acp-23-15325-2023Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.5194/acp-23-15325-2023Direct OA link when available
- Concepts
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Cloud condensation nuclei, Supersaturation, Particle (ecology), Condensation, Particle number, Chemistry, Analytical Chemistry (journal), Aerosol, Environmental chemistry, Meteorology, Thermodynamics, Physics, Organic chemistry, Geology, Oceanography, Volume (thermodynamics)Top concepts (fields/topics) attached by OpenAlex
- Cited by
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7Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 3, 2023: 1Per-year citation counts (last 5 years)
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144Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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