Ionic Tunability of Conjugated Polyelectrolyte Solutions Article Swipe
Scott P. O. Danielsen
,
Brittany J. Thompson
,
Glenn H. Fredrickson
,
Thuc‐Quyen Nguyen
,
Guillermo C. Bazan
,
Rachel A. Segalman
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acs.macromol.2c00178
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acs.macromol.2c00178
Conjugated polyelectrolytes (CPEs), which combine a π-conjugated polymer backbone with pendant ionic functionalities, offer an opportunity for electrostatic control of materials properties. In this work, the mesoscale morphology and physical properties of a high-mobility conjugated polyelectrolyte are tuned by the addition of salt, variation of the charge-compensating counterion, and complexation with an oppositely charged polyelectrolyte containing the same π-conjugated backbone. In systems with a single polyelectrolyte species, added ions screen the electrostatic repulsions stabilizing the gel-phase, resulting in the dissolution of ionic cross-links and hydrophobic collapse. Further, exchanging the charge compensating counterion is found to enable finer structural control of the solution behavior and modulation of the self-doping behavior. Finally, novel CPE–CPE complexes resulting in dense solutions and gels of semiconductive material are produced by combination of oppositely charged polyelectrolytes. Such concentrated CPE formulations should be useful materials for mixed electronic–ionic conduction and pseudocapacitative energy storage.
Related Topics
Concepts
Polyelectrolyte
Counterion
Ionic bonding
Polymer
Conjugated system
Dissolution
Chemical engineering
Chemical physics
Polyelectrolyte adsorption
Chemistry
Ionic conductivity
Phase (matter)
Ion
Materials science
Electrolyte
Polymer chemistry
Organic chemistry
Physical chemistry
Electrode
Engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.macromol.2c00178
- OA Status
- green
- Cited By
- 17
- References
- 110
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4225015697
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4225015697Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.macromol.2c00178Digital Object Identifier
- Title
-
Ionic Tunability of Conjugated Polyelectrolyte SolutionsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-04-26Full publication date if available
- Authors
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Scott P. O. Danielsen, Brittany J. Thompson, Glenn H. Fredrickson, Thuc‐Quyen Nguyen, Guillermo C. Bazan, Rachel A. SegalmanList of authors in order
- Landing page
-
https://doi.org/10.1021/acs.macromol.2c00178Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://www.osti.gov/biblio/1864920Direct OA link when available
- Concepts
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Polyelectrolyte, Counterion, Ionic bonding, Polymer, Conjugated system, Dissolution, Chemical engineering, Chemical physics, Polyelectrolyte adsorption, Chemistry, Ionic conductivity, Phase (matter), Ion, Materials science, Electrolyte, Polymer chemistry, Organic chemistry, Physical chemistry, Electrode, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
17Total citation count in OpenAlex
- Citations by year (recent)
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2025: 5, 2024: 1, 2023: 8, 2022: 3Per-year citation counts (last 5 years)
- References (count)
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110Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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