Isotopic fractionation as in-situ sensor of subsurface reactive flow and precursor for rock failure Article Swipe
Anastasia Ilgen
,
Robert Choens
,
Andrew W. Knight
,
Jacob Harvey
,
Mario Iglesias Martínez
,
Hongkyu Yoon
,
Jennifer Wilson
,
Melissa Mills
,
Qiaoyi Wang
,
Michael Gruenwald
,
Pania Newell
,
Louis Schuler
,
Haley and Davis
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.2172/1820526
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.2172/1820526
Greater utilization of subsurface reservoirs perturbs in-situ chemical-mechanical conditions with wide ranging consequences from decreased performance to project failure. Understanding the chemical precursors to rock deformation is critical to reducing the risks of these activities. To address this need, we investigated the coupled flow-dissolution- precipitation-adsorption reactions involving calcite and environmentally-relevant solid phases. Experimentally, we quantified (1) stable isotope fractionation processes for strontium during calcite nucleation and growth, and during reactive fluid flow; (2) consolidation behavior of calcite assemblages in the common brines. Numerically, we quantified water weakening of calcite using molecular dynamics simulations; and quantified the impact of calcite dissolution rate on macroscopic fracturing using finite element models. With microfluidic experiments and modeling, we show the effect of local flow fields on the dissolution kinetics of calcite. Taken together across a wide range of scales and methods, our studies allow us to separate the effects of reaction, flow, and transport, on calcite fracturing and the evolution of strontium isotopic signatures in the reactive fluids.
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- OA Status
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- OpenAlex ID
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All OpenAlex metadata
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https://doi.org/10.2172/1820526Digital Object Identifier
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Isotopic fractionation as in-situ sensor of subsurface reactive flow and precursor for rock failureWork title
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reportOpenAlex work type
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enPrimary language
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2021Year of publication
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2021-09-01Full publication date if available
- Authors
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Anastasia Ilgen, Robert Choens, Andrew W. Knight, Jacob Harvey, Mario Iglesias Martínez, Hongkyu Yoon, Jennifer Wilson, Melissa Mills, Qiaoyi Wang, Michael Gruenwald, Pania Newell, Louis Schuler, Haley and DavisList of authors in order
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https://doi.org/10.2172/1820526Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/1820526Direct OA link when available
- Concepts
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Calcite, Dissolution, Strontium, Nucleation, Geology, Mineralogy, Chemical engineering, Chemistry, Engineering, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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