Kinetics Manipulation Enabled by Solubility Control Toward 19% Organic Solar Cells via Compatible Air Coating Article Swipe
Yongwen Lang
,
Ying Zhang
,
Hao Xia
,
Kuan Liu
,
Yúang Fu
,
Liang Han
,
W.K. Fong
,
Dongyang Li
,
Miao Zhang
,
Wai‐Yeung Wong
,
Xinhui Lu
,
Tiangang Yang
,
Feng He
,
Yang Yang
,
Gang Li
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202420096
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202420096
Blade coating is a promising tool for upscaling organic solar cells (OSCs). However, the performances of blade‐coated OSCs still lag behind their spin‐coated counterparts, limiting their competitive edge towards commercialization. One of the main reasons is that controlling the film aggregation kinetics and morphology becomes challenging during the transition from spin coating to blade coating, especially when using high boiling point solvents, which can result in excessive aggregation. Therefore, a deeper understanding and appraisal of film formation kinetics influenced by coating methods is crucial. In this work, it is demonstrated that ink solubility tuning by incorporating a twisted third component (BTP‐4Cl) can induce rapid crystallization behavior and promote fine phase separation between the donor polymer (PM6) and the acceptor (BTP‐eC9) in blade coating. As a result, a high power conversion efficiency (PCE) of 19.67% is obtained in OSCs (0.04 cm 2 ), one of the state‐of‐the‐art efficiencies among the reported blade‐coated OSCs (19.76% for the spin‐coated devices). In addition, it is found that the inhibited phase aggregation contributes to enhancing the light stability of the device. This strategy offered novel insights into the effectiveness of solubility‐tuning approaches for achieving highly efficient and stable OSCs under open‐air coating conditions.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202420096
- OA Status
- green
- Cited By
- 8
- References
- 72
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4407907979
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4407907979Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202420096Digital Object Identifier
- Title
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Kinetics Manipulation Enabled by Solubility Control Toward 19% Organic Solar Cells via Compatible Air CoatingWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-02-23Full publication date if available
- Authors
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Yongwen Lang, Ying Zhang, Hao Xia, Kuan Liu, Yúang Fu, Liang Han, W.K. Fong, Dongyang Li, Miao Zhang, Wai‐Yeung Wong, Xinhui Lu, Tiangang Yang, Feng He, Yang Yang, Gang LiList of authors in order
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https://doi.org/10.1002/adma.202420096Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
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https://www.ncbi.nlm.nih.gov/pmc/articles/11983249Direct OA link when available
- Concepts
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Materials science, Solubility, Coating, Kinetics, Chemical engineering, Organic solar cell, Nanotechnology, Organic chemistry, Polymer, Composite material, Chemistry, Physics, Engineering, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
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8Total citation count in OpenAlex
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2025: 8Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.solubility | 93 |
| abstract_inverted_index.transition | 49 |
| abstract_inverted_index.(BTP‐4Cl) | 101 |
| abstract_inverted_index.(BTP‐eC9) | 120 |
| abstract_inverted_index.aggregation | 41, 167 |
| abstract_inverted_index.challenging | 46 |
| abstract_inverted_index.competitive | 27 |
| abstract_inverted_index.conditions. | 198 |
| abstract_inverted_index.contributes | 168 |
| abstract_inverted_index.controlling | 38 |
| abstract_inverted_index.aggregation. | 68 |
| abstract_inverted_index.demonstrated | 90 |
| abstract_inverted_index.efficiencies | 147 |
| abstract_inverted_index.performances | 15 |
| abstract_inverted_index.counterparts, | 24 |
| abstract_inverted_index.effectiveness | 184 |
| abstract_inverted_index.incorporating | 96 |
| abstract_inverted_index.spin‐coated | 23, 156 |
| abstract_inverted_index.understanding | 72 |
| abstract_inverted_index.blade‐coated | 17, 151 |
| abstract_inverted_index.crystallization | 105 |
| abstract_inverted_index.commercialization. | 30 |
| abstract_inverted_index.solubility‐tuning | 186 |
| abstract_inverted_index.state‐of‐the‐art | 146 |
| cited_by_percentile_year.max | 99 |
| cited_by_percentile_year.min | 98 |
| countries_distinct_count | 3 |
| institutions_distinct_count | 15 |
| citation_normalized_percentile.value | 0.98176319 |
| citation_normalized_percentile.is_in_top_1_percent | True |
| citation_normalized_percentile.is_in_top_10_percent | True |