Latent heat induced rotation limited aggregation in 2D ice nanocrystals Article Swipe
Pantelis Bampoulis
,
Martin Herman Siekman
,
E. Stefan Kooij
,
Detlef Lohse
,
Harold J. W. Zandvliet
,
Bene Poelsema
·
YOU?
·
· 2015
· Open Access
·
· DOI: https://doi.org/10.1063/1.4926467
YOU?
·
· 2015
· Open Access
·
· DOI: https://doi.org/10.1063/1.4926467
The basic science responsible for the fascinating shapes of ice crystals and snowflakes is still not understood. Insufficient knowledge of the interaction potentials and the lack of relevant experimental access to the growth process are to blame for this failure. Here, we study the growth of fractal nanostructures in a two-dimensional (2D) system, intercalated between mica and graphene. Based on our scanning tunneling spectroscopy data, we provide compelling evidence that these fractals are 2D ice. They grow while they are in material contact with the atmosphere at 20 °C and without significant thermal contact to the ambient. The growth is studied in situ, in real time and space at the nanoscale. We find that the growing 2D ice nanocrystals assume a fractal shape, which is conventionally attributed to Diffusion Limited Aggregation (DLA). However, DLA requires a low mass density mother phase, in contrast to the actual currently present high mass density mother phase. Latent heat effects and consequent transport of heat and molecules are found to be key ingredients for understanding the evolution of the snow (ice) flakes. We conclude that not the local availability of water molecules (DLA), but rather them having the locally required orientation is the key factor for incorporation into the 2D ice nanocrystal. In combination with the transport of latent heat, we attribute the evolution of fractal 2D ice nanocrystals to local temperature dependent rotation limited aggregation. The ice growth occurs under extreme supersaturation, i.e., the conditions closely resemble the natural ones for the growth of complex 2D snow (ice) flakes and we consider our findings crucial for solving the “perennial” snow (ice) flake enigma.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1063/1.4926467
- https://aip.scitation.org/doi/pdf/10.1063/1.4926467
- OA Status
- bronze
- Cited By
- 36
- References
- 37
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W1483248666
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W1483248666Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1063/1.4926467Digital Object Identifier
- Title
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Latent heat induced rotation limited aggregation in 2D ice nanocrystalsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2015Year of publication
- Publication date
-
2015-07-15Full publication date if available
- Authors
-
Pantelis Bampoulis, Martin Herman Siekman, E. Stefan Kooij, Detlef Lohse, Harold J. W. Zandvliet, Bene PoelsemaList of authors in order
- Landing page
-
https://doi.org/10.1063/1.4926467Publisher landing page
- PDF URL
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https://aip.scitation.org/doi/pdf/10.1063/1.4926467Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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bronzeOpen access status per OpenAlex
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https://aip.scitation.org/doi/pdf/10.1063/1.4926467Direct OA link when available
- Concepts
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Chemical physics, Snowflake, Ice crystals, Materials science, Latent heat, Nanocrystal, Nanotechnology, Snow, Chemistry, Physics, Thermodynamics, MeteorologyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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36Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2, 2024: 1, 2023: 1, 2022: 4, 2021: 4Per-year citation counts (last 5 years)
- References (count)
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37Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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