Lattice Oxygen Redox Dynamics in Zeolite‐Encapsulated CsPbBr3 Perovskite OER Electrocatalysts Article Swipe
Xiangrong Ren
,
Yiyue Zhai
,
Na Yang
,
Bolun Wang
,
Shengzhong Liu
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202412679
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202412679
Understanding the oxygen evolution reaction (OER) mechanism is pivotal for improving the overall efficiency of water electrolysis. Despite methylammonium lead halide perovskites (MAPbX 3 ) have shown promising OER performance due to their soft‐lattice nature that allows lattice‐oxygen oxidation of active α‐PbO 2 layer surface, the role of A‐site MA or X‐site elements in the electrochemical reconstruction and OER mechanisms has yet to be explored. Here, it is demonstrated that the OER mechanism of perovskite@zeolite composites is intrinsically dominated by the A‐site group of lead‐halide perovskites, while the type of X‐site halogen is crucial for the reconstruction kinetics of the composites. Using CsPbBr x I 3‐ x @AlPO‐5 ( x = 0, 1, 2, 3) as a model OER catalyst, it is found that the CsPbBr 3 @AlPO‐5 behaves oxygen‐intercalation pseudocapacitance during surface restructuring due to absence of halogen‐ion migration and phase separation in the CsPbBr 3 , achieving a larger diffusion rate of OH − within the core‐shell structure. Moreover, distinct from the single‐metal‐site mechanism of MAPbBr 3 @AlPO‐5, experimental and theoretical investigations reveal that the soft lattice nature of CsPbBr 3 triggers the oxygen‐vacancy‐site mechanism via the CsPbBr 3 /α‐PbO 2 interface, resulting in excellent OER performance. Owing to the variety and easy tailoring of lead‐halide perovskite compositions, these findings pave a way for the development of novel perovskite@zeolite type catalysts for efficient oxygen electrocatalysis.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/advs.202412679
- OA Status
- gold
- Cited By
- 9
- References
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- Related Works
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- OpenAlex ID
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https://openalex.org/W4406222609Canonical identifier for this work in OpenAlex
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https://doi.org/10.1002/advs.202412679Digital Object Identifier
- Title
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Lattice Oxygen Redox Dynamics in Zeolite‐Encapsulated CsPbBr3 Perovskite OER ElectrocatalystsWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-01-09Full publication date if available
- Authors
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Xiangrong Ren, Yiyue Zhai, Na Yang, Bolun Wang, Shengzhong LiuList of authors in order
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https://doi.org/10.1002/advs.202412679Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.1002/advs.202412679Direct OA link when available
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Oxygen evolution, Perovskite (structure), Materials science, Halide, Electrocatalyst, Catalysis, Zeolite, Inorganic chemistry, Chemistry, Chemical engineering, Electrochemistry, Physical chemistry, Electrode, Crystallography, Engineering, BiochemistryTop concepts (fields/topics) attached by OpenAlex
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9Total citation count in OpenAlex
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2025: 9Per-year citation counts (last 5 years)
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