Layer modulating and electrical properties in acceptor-doped Sr5Nb5O17 ceramic with perovskite layer structure Article Swipe
Xiaoxu Duan
,
Jungu Xu
,
Xianfeng Yang
,
He Xiao-Ling
,
Cheng Wang
,
Laijun Liu
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.20517/microstructures.2024.132
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.20517/microstructures.2024.132
Perovskite layer structured (PLS) oxides exhibit some novel physical properties, such as ultrahigh-temperature piezoelectricity, semiconductivity, and oxygen ionic transport. However, synthesizing 5-layer PLS oxides, such as Sr5Nb5O17 ceramics, using traditional solid-state reaction methods is challenging due to their low phase stability. In this study, we propose a new strategy to construct a 5-layer structure from a 4-layer structure. Specifically, Ga-doped Sr5Nb4.444Ga0.556O16.944 (5-SNGO), an iso-structural material to Sr5Nb5O17, was synthesized via a solid-phase reaction. The original design involved co-doping Ga and Mo at the Nb site of the 4-layer parent material Sr2Nb2O7 (4-SNO). However, it was found that only Ga was successfully incorporated into the structure, while Mo remained as SrMoO4, which was subsequently removed by washing with dilute sulfuric acid. X-ray diffraction, transmission electron microscopy, and second-harmonic generation analysis confirmed that the synthesized 5-SNGO ceramic exhibits a 5-layer structure with a noncentrosymmetric space group. The material demonstrated a frequency-independent dielectric permittivity of 60 above 1 kHz. Impedance spectroscopy revealed a very high resistivity of 1.95 × 105 Ω·cm at 900 °C, along with Debye-like dielectric relaxation exhibiting thermal activation behavior. This study presents a novel synthesis approach for constructing 5-layer PLS oxides from a 4-layer structure and provides insights into their structural evolution and electrical properties.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.20517/microstructures.2024.132
- https://f.oaes.cc/xmlpdf/63f01b1a-5e3a-41be-8488-1e5e68f2d358/microstructures40132.pdf
- OA Status
- hybrid
- Cited By
- 1
- References
- 38
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4409609885
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https://openalex.org/W4409609885Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.20517/microstructures.2024.132Digital Object Identifier
- Title
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Layer modulating and electrical properties in acceptor-doped Sr5Nb5O17 ceramic with perovskite layer structureWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-04-21Full publication date if available
- Authors
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Xiaoxu Duan, Jungu Xu, Xianfeng Yang, He Xiao-Ling, Cheng Wang, Laijun LiuList of authors in order
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https://doi.org/10.20517/microstructures.2024.132Publisher landing page
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https://f.oaes.cc/xmlpdf/63f01b1a-5e3a-41be-8488-1e5e68f2d358/microstructures40132.pdfDirect link to full text PDF
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://f.oaes.cc/xmlpdf/63f01b1a-5e3a-41be-8488-1e5e68f2d358/microstructures40132.pdfDirect OA link when available
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Materials science, Perovskite (structure), Acceptor, Ceramic, Doping, Layer (electronics), Mineralogy, Optoelectronics, Condensed matter physics, Crystallography, Composite material, Chemistry, PhysicsTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2025: 1Per-year citation counts (last 5 years)
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38Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.ceramic | 134 |
| abstract_inverted_index.exhibit | 5 |
| abstract_inverted_index.methods | 32 |
| abstract_inverted_index.oxides, | 23 |
| abstract_inverted_index.propose | 45 |
| abstract_inverted_index.removed | 113 |
| abstract_inverted_index.thermal | 177 |
| abstract_inverted_index.washing | 115 |
| abstract_inverted_index.(4-SNO). | 91 |
| abstract_inverted_index.Ga-doped | 59 |
| abstract_inverted_index.However, | 19, 92 |
| abstract_inverted_index.Sr2Nb2O7 | 90 |
| abstract_inverted_index.analysis | 128 |
| abstract_inverted_index.approach | 186 |
| abstract_inverted_index.electron | 123 |
| abstract_inverted_index.exhibits | 135 |
| abstract_inverted_index.insights | 198 |
| abstract_inverted_index.involved | 76 |
| abstract_inverted_index.material | 64, 89, 145 |
| abstract_inverted_index.original | 74 |
| abstract_inverted_index.physical | 8 |
| abstract_inverted_index.presents | 182 |
| abstract_inverted_index.provides | 197 |
| abstract_inverted_index.reaction | 31 |
| abstract_inverted_index.remained | 107 |
| abstract_inverted_index.revealed | 158 |
| abstract_inverted_index.strategy | 48 |
| abstract_inverted_index.sulfuric | 118 |
| abstract_inverted_index.(5-SNGO), | 61 |
| abstract_inverted_index.Impedance | 156 |
| abstract_inverted_index.Sr5Nb5O17 | 26 |
| abstract_inverted_index.behavior. | 179 |
| abstract_inverted_index.ceramics, | 27 |
| abstract_inverted_index.co-doping | 77 |
| abstract_inverted_index.confirmed | 129 |
| abstract_inverted_index.construct | 50 |
| abstract_inverted_index.evolution | 202 |
| abstract_inverted_index.reaction. | 72 |
| abstract_inverted_index.structure | 53, 138, 195 |
| abstract_inverted_index.synthesis | 185 |
| abstract_inverted_index.Debye-like | 173 |
| abstract_inverted_index.Perovskite | 0 |
| abstract_inverted_index.Sr5Nb5O17, | 66 |
| abstract_inverted_index.activation | 178 |
| abstract_inverted_index.dielectric | 149, 174 |
| abstract_inverted_index.electrical | 204 |
| abstract_inverted_index.exhibiting | 176 |
| abstract_inverted_index.generation | 127 |
| abstract_inverted_index.relaxation | 175 |
| abstract_inverted_index.stability. | 40 |
| abstract_inverted_index.structural | 201 |
| abstract_inverted_index.structure, | 104 |
| abstract_inverted_index.structure. | 57 |
| abstract_inverted_index.structured | 2 |
| abstract_inverted_index.transport. | 18 |
| abstract_inverted_index.challenging | 34 |
| abstract_inverted_index.microscopy, | 124 |
| abstract_inverted_index.properties, | 9 |
| abstract_inverted_index.properties. | 205 |
| abstract_inverted_index.resistivity | 162 |
| abstract_inverted_index.solid-phase | 71 |
| abstract_inverted_index.solid-state | 30 |
| abstract_inverted_index.synthesized | 68, 132 |
| abstract_inverted_index.traditional | 29 |
| abstract_inverted_index.constructing | 188 |
| abstract_inverted_index.demonstrated | 146 |
| abstract_inverted_index.diffraction, | 121 |
| abstract_inverted_index.incorporated | 101 |
| abstract_inverted_index.permittivity | 150 |
| abstract_inverted_index.spectroscopy | 157 |
| abstract_inverted_index.subsequently | 112 |
| abstract_inverted_index.successfully | 100 |
| abstract_inverted_index.synthesizing | 20 |
| abstract_inverted_index.transmission | 122 |
| abstract_inverted_index.Specifically, | 58 |
| abstract_inverted_index.iso-structural | 63 |
| abstract_inverted_index.second-harmonic | 126 |
| abstract_inverted_index.piezoelectricity, | 13 |
| abstract_inverted_index.semiconductivity, | 14 |
| abstract_inverted_index.noncentrosymmetric | 141 |
| abstract_inverted_index.frequency-independent | 148 |
| abstract_inverted_index.ultrahigh-temperature | 12 |
| abstract_inverted_index.Sr5Nb4.444Ga0.556O16.944 | 60 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 91 |
| countries_distinct_count | 0 |
| institutions_distinct_count | 6 |
| citation_normalized_percentile.value | 0.67196328 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |