Li 2 MnCl 4 for neutron detection: tailoring red emission via doping Article Swipe
K Křehlíková
,
V Vaněček
,
R Král
,
P Průša
,
R Kučerková
,
V Babin
,
J Rohlíček
,
K Rubešová
,
M Nikl
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1088/1742-6596/3157/1/012007
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1088/1742-6596/3157/1/012007
In this work, we report on the growth of red-emitting lithium manganese(II) chloride (Li 2 MnCl 4 , LMC), a potential candidate for thermal neutron detection. The doping of Li 2 MnCl 4 was proposed to optimize scintillation efficiency and three single crystals of Li 2 MnCl 4 :Sm 2+ , Li 2 MnCl 4 :Ti 3+ , and Li 2 MnCl 4 :In + were grown by miniaturized vertical Bridgman method (mVB). While crystal growth was successful, the results from optical measurements indicated limited achievement in the optimization of luminescence properties. Ti 3+ incorporation into the Li 2 MnCl 4 lattice was highly uncertain, as neither the absorbance data nor the radioluminescence (RL) spectrum exhibited bands corresponding to the Ti 3+ 2 E → 2 T 2 radiative transition. In the case of Sm 2+ - and In +_ doping, the RL efficiencies achieved only 3.39 and 2.14% of the bismuth germanate (Bi 4 Ge 3 O 12 , BGO) reference sample, respectively. Since the Li 2 MnCl 4 :Sm 2+ photoluminescence (PL) spectra revealed line emissions corresponding to the Sm 2+ forbidden 4 f 6 → 4 f 6 transitions, the temperature-dependent PL was measured. At higher temperatures (specifically, from 437 K), the broad emission of the 4 f 5 5 d → 4 f 6 transition dominated, which indicated the thermal population of the 5 d state.
Related Topics
Concepts
Photoluminescence
Radioluminescence
Analytical Chemistry (journal)
Doping
Luminescence
Emission spectrum
Chemistry
Materials science
Dopant
Population
Single crystal
Crystal (programming language)
Spectral line
Scintillation
Chalcogenide
Bismuth germanate
Neutron
Excitation
Neutron temperature
Crystal structure
Stimulated emission
Lithium (medication)
Absorbance
Nuclear chemistry
Absorption spectroscopy
Inorganic chemistry
Metadata
- Type
- article
- Landing Page
- https://doi.org/10.1088/1742-6596/3157/1/012007
- OA Status
- diamond
- References
- 17
- OpenAlex ID
- https://openalex.org/W7111281882
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W7111281882Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1088/1742-6596/3157/1/012007Digital Object Identifier
- Title
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Li 2 MnCl 4 for neutron detection: tailoring red emission via dopingWork title
- Type
-
articleOpenAlex work type
- Publication year
-
2025Year of publication
- Publication date
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2025-12-01Full publication date if available
- Authors
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K Křehlíková, V Vaněček, R Král, P Průša, R Kučerková, V Babin, J Rohlíček, K Rubešová, M NiklList of authors in order
- Landing page
-
https://doi.org/10.1088/1742-6596/3157/1/012007Publisher landing page
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YesWhether a free full text is available
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diamondOpen access status per OpenAlex
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https://doi.org/10.1088/1742-6596/3157/1/012007Direct OA link when available
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Photoluminescence, Radioluminescence, Analytical Chemistry (journal), Doping, Luminescence, Emission spectrum, Chemistry, Materials science, Dopant, Population, Single crystal, Crystal (programming language), Spectral line, Scintillation, Chalcogenide, Bismuth germanate, Neutron, Excitation, Neutron temperature, Crystal structure, Stimulated emission, Lithium (medication), Absorbance, Nuclear chemistry, Absorption spectroscopy, Inorganic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- References (count)
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17Number of works referenced by this work
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| abstract_inverted_index.f | 186, 190, 211, 217 |
| abstract_inverted_index.+_ | 140 |
| abstract_inverted_index.12 | 159 |
| abstract_inverted_index.2+ | 50, 136, 172, 183 |
| abstract_inverted_index.3+ | 57, 94, 122 |
| abstract_inverted_index.At | 198 |
| abstract_inverted_index.Ge | 156 |
| abstract_inverted_index.In | 1, 131, 139 |
| abstract_inverted_index.Li | 30, 45, 52, 60, 98, 167 |
| abstract_inverted_index.PL | 195 |
| abstract_inverted_index.RL | 143 |
| abstract_inverted_index.Sm | 135, 182 |
| abstract_inverted_index.Ti | 93, 121 |
| abstract_inverted_index.as | 106 |
| abstract_inverted_index.by | 68 |
| abstract_inverted_index.in | 87 |
| abstract_inverted_index.of | 9, 29, 44, 90, 134, 150, 208, 226 |
| abstract_inverted_index.on | 6 |
| abstract_inverted_index.to | 36, 119, 180 |
| abstract_inverted_index.we | 4 |
| abstract_inverted_index.(Bi | 154 |
| abstract_inverted_index.(Li | 14 |
| abstract_inverted_index.437 | 203 |
| abstract_inverted_index.:In | 64 |
| abstract_inverted_index.:Sm | 49, 171 |
| abstract_inverted_index.:Ti | 56 |
| abstract_inverted_index.K), | 204 |
| abstract_inverted_index.The | 27 |
| abstract_inverted_index.and | 40, 59, 138, 148 |
| abstract_inverted_index.for | 23 |
| abstract_inverted_index.nor | 111 |
| abstract_inverted_index.the | 7, 79, 88, 97, 108, 112, 120, 132, 142, 151, 166, 181, 193, 205, 209, 223, 227 |
| abstract_inverted_index.was | 34, 77, 103, 196 |
| abstract_inverted_index.→ | 125, 188, 215 |
| abstract_inverted_index.(PL) | 174 |
| abstract_inverted_index.(RL) | 114 |
| abstract_inverted_index.3.39 | 147 |
| abstract_inverted_index.BGO) | 161 |
| abstract_inverted_index.MnCl | 16, 32, 47, 54, 62, 100, 169 |
| abstract_inverted_index.case | 133 |
| abstract_inverted_index.data | 110 |
| abstract_inverted_index.from | 81, 202 |
| abstract_inverted_index.into | 96 |
| abstract_inverted_index.line | 177 |
| abstract_inverted_index.only | 146 |
| abstract_inverted_index.this | 2 |
| abstract_inverted_index.were | 66 |
| abstract_inverted_index.2.14% | 149 |
| abstract_inverted_index.LMC), | 19 |
| abstract_inverted_index.Since | 165 |
| abstract_inverted_index.While | 74 |
| abstract_inverted_index.bands | 117 |
| abstract_inverted_index.broad | 206 |
| abstract_inverted_index.grown | 67 |
| abstract_inverted_index.three | 41 |
| abstract_inverted_index.which | 221 |
| abstract_inverted_index.work, | 3 |
| abstract_inverted_index.(mVB). | 73 |
| abstract_inverted_index.doping | 28 |
| abstract_inverted_index.growth | 8, 76 |
| abstract_inverted_index.higher | 199 |
| abstract_inverted_index.highly | 104 |
| abstract_inverted_index.method | 72 |
| abstract_inverted_index.report | 5 |
| abstract_inverted_index.single | 42 |
| abstract_inverted_index.state. | 230 |
| abstract_inverted_index.bismuth | 152 |
| abstract_inverted_index.crystal | 75 |
| abstract_inverted_index.doping, | 141 |
| abstract_inverted_index.lattice | 102 |
| abstract_inverted_index.limited | 85 |
| abstract_inverted_index.lithium | 11 |
| abstract_inverted_index.neither | 107 |
| abstract_inverted_index.neutron | 25 |
| abstract_inverted_index.optical | 82 |
| abstract_inverted_index.results | 80 |
| abstract_inverted_index.sample, | 163 |
| abstract_inverted_index.spectra | 175 |
| abstract_inverted_index.thermal | 24, 224 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.Bridgman | 71 |
| abstract_inverted_index.achieved | 145 |
| abstract_inverted_index.chloride | 13 |
| abstract_inverted_index.crystals | 43 |
| abstract_inverted_index.emission | 207 |
| abstract_inverted_index.optimize | 37 |
| abstract_inverted_index.proposed | 35 |
| abstract_inverted_index.revealed | 176 |
| abstract_inverted_index.spectrum | 115 |
| abstract_inverted_index.vertical | 70 |
| abstract_inverted_index.candidate | 22 |
| abstract_inverted_index.emissions | 178 |
| abstract_inverted_index.exhibited | 116 |
| abstract_inverted_index.forbidden | 184 |
| abstract_inverted_index.germanate | 153 |
| abstract_inverted_index.indicated | 84, 222 |
| abstract_inverted_index.measured. | 197 |
| abstract_inverted_index.potential | 21 |
| abstract_inverted_index.radiative | 129 |
| abstract_inverted_index.reference | 162 |
| abstract_inverted_index.absorbance | 109 |
| abstract_inverted_index.detection. | 26 |
| abstract_inverted_index.dominated, | 220 |
| abstract_inverted_index.efficiency | 39 |
| abstract_inverted_index.population | 225 |
| abstract_inverted_index.transition | 219 |
| abstract_inverted_index.uncertain, | 105 |
| abstract_inverted_index.achievement | 86 |
| abstract_inverted_index.properties. | 92 |
| abstract_inverted_index.successful, | 78 |
| abstract_inverted_index.transition. | 130 |
| abstract_inverted_index.efficiencies | 144 |
| abstract_inverted_index.luminescence | 91 |
| abstract_inverted_index.measurements | 83 |
| abstract_inverted_index.miniaturized | 69 |
| abstract_inverted_index.optimization | 89 |
| abstract_inverted_index.red-emitting | 10 |
| abstract_inverted_index.temperatures | 200 |
| abstract_inverted_index.transitions, | 192 |
| abstract_inverted_index.corresponding | 118, 179 |
| abstract_inverted_index.incorporation | 95 |
| abstract_inverted_index.manganese(II) | 12 |
| abstract_inverted_index.respectively. | 164 |
| abstract_inverted_index.scintillation | 38 |
| abstract_inverted_index.(specifically, | 201 |
| abstract_inverted_index.photoluminescence | 173 |
| abstract_inverted_index.radioluminescence | 113 |
| abstract_inverted_index.temperature-dependent | 194 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 9 |
| citation_normalized_percentile.value | 0.82487887 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |