Light-Induced Currents at Domain Walls in Multiferroic BiFeO3 Article Swipe
YOU?
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· 2019
· Open Access
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· DOI: https://doi.org/10.1021/acs.nanolett.9b03484
Multiferroic BiFeO3 (BFO) films with spontaneously formed periodic stripe domains can generate above-gap open circuit voltages under visible light illumination; nevertheless the underlying mechanism behind this intriguing optoelectronic response has not been understood to date. Here, we make contact-free measurements of light-induced currents in epitaxial BFO films via detecting terahertz radiation emanated by these currents, enabling a direct probe of the intrinsic charge separation mechanisms along with quantitative measurements of the current amplitudes and their directions. In the periodic stripe samples, we find that the net photocurrent is dominated by the charge separation across the domain walls, whereas in the monodomain samples the photovoltaic response arises from a bulk shift current associated with the non-centrosymmetry of the crystal. The peak current amplitude driven by the charge separation at the domain walls is found to be 2 orders of magnitude higher than the bulk shift current response, indicating the prominent role of domain walls acting as nanoscale junctions to efficiently separate photogenerated charges in the stripe domain BFO films. These findings show that domain-wall-engineered BFO thin films offer exciting prospects for ferroelectric-based optoelectronics, as well as bias-free strong terahertz emitters.
Related Topics
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.nanolett.9b03484
- OA Status
- green
- Cited By
- 41
- References
- 37
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2990427924
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W2990427924Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1021/acs.nanolett.9b03484Digital Object Identifier
- Title
-
Light-Induced Currents at Domain Walls in Multiferroic BiFeO3Work title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2019Year of publication
- Publication date
-
2019-11-20Full publication date if available
- Authors
-
Burak Güzeltürk, Antonio B. Mei, Lei Zhang, Liang Z. Tan, C. Donahue, Anisha G. Singh, Darrell G. Schlom, Lane W. Martin, Aaron M. LindenbergList of authors in order
- Landing page
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https://doi.org/10.1021/acs.nanolett.9b03484Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://www.osti.gov/biblio/1604721Direct OA link when available
- Concepts
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Photocurrent, Materials science, Multiferroics, Ferroelectricity, Domain wall (magnetism), Condensed matter physics, Optoelectronics, Amplitude, Terahertz radiation, Thin film, Optics, Nanotechnology, Physics, Dielectric, Quantum mechanics, Magnetic field, MagnetizationTop concepts (fields/topics) attached by OpenAlex
- Cited by
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41Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2, 2024: 4, 2023: 10, 2022: 6, 2021: 13Per-year citation counts (last 5 years)
- References (count)
-
37Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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