Light-Induced Structural Dynamics and Charge Transport in Layered Halide Perovskite Thin Films Article Swipe
Hsinhan Tsai
,
Dibyajyoti Ghosh
,
Eli Diego Kinigstein
,
Bogdan Dryzhakov
,
Honora Driscoll
,
Magdalena Owczarek
,
Bin Hu
,
Xiaoyi Zhang
,
Sergei Tretiak
,
Wanyi Nie
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/acs.nanolett.2c03403
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/acs.nanolett.2c03403
The dynamic nature of the metal halide perovskite lattice upon photoexcitation plays a vital role in their properties. Here we report an observation of light-induced structure dynamics in quasi-2D Ruddlesden-Popper phase perovskite thin films and its impact on the carrier transport properties. By a time-resolved X-ray scattering technique, we observe a rapid lattice expansion upon photoexcitation, followed by a slow relaxation over the course of 100 ns in the dark. Theoretical modeling suggests that the expansion originates from the lattice's thermal fluctuations caused by photon energy deposition. Power dependent optical spectroscopy and photoconductivity indicate that high laser powers triggered a strong local structural disorder, which increased the charge dissociation activation energy that results in localized transport. Our study investigates the impact of laser energy deposition on the lattices and the subsequent carrier transport properties, that are relevant to device operations.
Related Topics
Concepts
Photoexcitation
Perovskite (structure)
Thin film
Chemical physics
Charge carrier
Materials science
Halide
Scattering
Dissociation (chemistry)
Condensed matter physics
Chemistry
Optoelectronics
Optics
Nanotechnology
Excited state
Atomic physics
Physical chemistry
Crystallography
Inorganic chemistry
Physics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.nanolett.2c03403
- OA Status
- green
- Cited By
- 11
- References
- 51
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4313537751
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4313537751Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.nanolett.2c03403Digital Object Identifier
- Title
-
Light-Induced Structural Dynamics and Charge Transport in Layered Halide Perovskite Thin FilmsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-01-05Full publication date if available
- Authors
-
Hsinhan Tsai, Dibyajyoti Ghosh, Eli Diego Kinigstein, Bogdan Dryzhakov, Honora Driscoll, Magdalena Owczarek, Bin Hu, Xiaoyi Zhang, Sergei Tretiak, Wanyi NieList of authors in order
- Landing page
-
https://doi.org/10.1021/acs.nanolett.2c03403Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://www.osti.gov/biblio/1909561Direct OA link when available
- Concepts
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Photoexcitation, Perovskite (structure), Thin film, Chemical physics, Charge carrier, Materials science, Halide, Scattering, Dissociation (chemistry), Condensed matter physics, Chemistry, Optoelectronics, Optics, Nanotechnology, Excited state, Atomic physics, Physical chemistry, Crystallography, Inorganic chemistry, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
11Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 3, 2024: 3, 2023: 5Per-year citation counts (last 5 years)
- References (count)
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51Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.expansion | 53, 75 |
| abstract_inverted_index.increased | 105 |
| abstract_inverted_index.lattice's | 79 |
| abstract_inverted_index.localized | 114 |
| abstract_inverted_index.structure | 25 |
| abstract_inverted_index.transport | 40, 132 |
| abstract_inverted_index.triggered | 98 |
| abstract_inverted_index.activation | 109 |
| abstract_inverted_index.deposition | 124 |
| abstract_inverted_index.originates | 76 |
| abstract_inverted_index.perovskite | 7, 31 |
| abstract_inverted_index.relaxation | 60 |
| abstract_inverted_index.scattering | 46 |
| abstract_inverted_index.structural | 102 |
| abstract_inverted_index.subsequent | 130 |
| abstract_inverted_index.technique, | 47 |
| abstract_inverted_index.transport. | 115 |
| abstract_inverted_index.Theoretical | 70 |
| abstract_inverted_index.deposition. | 86 |
| abstract_inverted_index.observation | 22 |
| abstract_inverted_index.operations. | 139 |
| abstract_inverted_index.properties, | 133 |
| abstract_inverted_index.properties. | 17, 41 |
| abstract_inverted_index.dissociation | 108 |
| abstract_inverted_index.fluctuations | 81 |
| abstract_inverted_index.investigates | 118 |
| abstract_inverted_index.spectroscopy | 90 |
| abstract_inverted_index.light-induced | 24 |
| abstract_inverted_index.time-resolved | 44 |
| abstract_inverted_index.photoexcitation | 10 |
| abstract_inverted_index.photoexcitation, | 55 |
| abstract_inverted_index.Ruddlesden-Popper | 29 |
| abstract_inverted_index.photoconductivity | 92 |
| cited_by_percentile_year.max | 98 |
| cited_by_percentile_year.min | 96 |
| corresponding_author_ids | https://openalex.org/A5082395322 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I1343871089, https://openalex.org/I4210127218 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.8600000143051147 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile.value | 0.8373507 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |