Light‐Controlled Nucleation and Shaping of Self‐Assembling Nanocomposites Article Swipe
Marloes H. Bistervels
,
M. Kamp
,
Hinco Schoenmaker
,
Albert M. Brouwer
,
Willem L. Noorduin
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202107843
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202107843
Controlling self‐assembly of nanocomposites is a fundamental challenge with exciting implications for next‐generation advanced functional materials. Precursors for composites can be generated photochemically, but limited insight in the underlying processes has hindered precise hands‐on guidance. In this study, light‐controlled nucleation and growth is demonstrated for self‐assembling composites according to precise user‐defined designs. Carbonate is generated photochemically with UV light to steer the precipitation of nanocomposites of barium carbonate nanocrystals and amorphous silica (BaCO 3 /SiO 2 ). Using a custom‐built optical setup, the self‐assembly process is controlled by optimizing the photogeneration, diffusion, reaction, and precipitation of the carbonate species, using the radius and intensity of the UV‐light irradiated area and reaction temperature. Exploiting this control, nucleation is induced and the contours and individual features of the growing composite are sculpted according to micrometer‐defined light patterns. Moreover, moving light patterns are exploited to create a constant carbonate concentration at the growth front to draw lines of nanocomposites with constant width over millimeters with micrometer precision. Light‐directed generation of local gradients opens previously unimaginable opportunities for guiding self‐assembly into functional materials.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202107843
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202107843
- OA Status
- hybrid
- Cited By
- 20
- References
- 28
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3215963327
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https://openalex.org/W3215963327Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202107843Digital Object Identifier
- Title
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Light‐Controlled Nucleation and Shaping of Self‐Assembling NanocompositesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
-
2021-12-02Full publication date if available
- Authors
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Marloes H. Bistervels, M. Kamp, Hinco Schoenmaker, Albert M. Brouwer, Willem L. NoorduinList of authors in order
- Landing page
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https://doi.org/10.1002/adma.202107843Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202107843Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202107843Direct OA link when available
- Concepts
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Materials science, Nanocomposite, Nucleation, Micrometer, Amorphous solid, Barium carbonate, Precipitation, Nanotechnology, Nanocrystal, Composite number, Chemical engineering, Composite material, Optics, Crystallography, Meteorology, Engineering, Physics, Organic chemistry, Chemistry, Raw materialTop concepts (fields/topics) attached by OpenAlex
- Cited by
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20Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 4, 2023: 7, 2022: 5, 2021: 1Per-year citation counts (last 5 years)
- References (count)
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28Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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