Lithiation‐Induced Defect Engineering to Promote Oxygen Evolution Reaction Article Swipe
Jingjie Liu
,
Mengting Zheng
,
Jiantao Li
,
Yifei Yuan
,
Chenghang Li
,
Shanqing Zhang
,
Lin Yang
,
Zhengyu Bai
,
Jun Lü
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202209753
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202209753
Exploring efficient electrocatalysts for oxygen evolution reaction (OER) is an urgent need to advance the development of sustainable energy conversion. Though defect engineering is considered an effective strategy to regulate catalyst activity for enhanced OER performance, the controllable synthesis of defective oxides electrocatalysts remains challenging. Here, oxygen defects are introduced into NiCo 2 O 4 nanorods by an electrochemical lithiation strategy. By tuning in situ lithiation potentials, the concentration of oxygen defects and the corresponding catalytic activity can be feasibly regulated. In addition, the relationship between the changes in the defect density and electronic structure and the lithiation cut‐off voltages is revealed. The results show that NiCo 2 O 4 nanorods undertook intercalation and two‐step conversion reaction, in which the lithiation‐induced conversion reaction gives rise to a CoO@NiO‐based structure with higher defect density and lower oxidation states. As a result, the defective CoO@NiO‐based catalyst exhibits exceptional OER activity with an overpotential of 270 mV at 10 mA cm −2 , which is about 74 mV below the pristine nanomaterials. This research proposes a novel strategy to explore high‐performance catalysts with structural stability and defect control.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adfm.202209753
- OA Status
- green
- Cited By
- 36
- References
- 50
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4310193727
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4310193727Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adfm.202209753Digital Object Identifier
- Title
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Lithiation‐Induced Defect Engineering to Promote Oxygen Evolution ReactionWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-11-28Full publication date if available
- Authors
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Jingjie Liu, Mengting Zheng, Jiantao Li, Yifei Yuan, Chenghang Li, Shanqing Zhang, Lin Yang, Zhengyu Bai, Jun LüList of authors in order
- Landing page
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https://doi.org/10.1002/adfm.202209753Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/2305385Direct OA link when available
- Concepts
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Overpotential, Oxygen evolution, Nanorod, Materials science, Catalysis, Non-blocking I/O, Nanomaterials, Intercalation (chemistry), Electrochemistry, Chemical engineering, Oxygen, Nanotechnology, Inorganic chemistry, Electrode, Physical chemistry, Chemistry, Engineering, Biochemistry, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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36Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 19, 2023: 14Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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