Long-Range Electron Transport Donor-Acceptor in Nonlinear Lattices Article Swipe
A. P. Chetverikov
,
W. Ebeling
,
Manuel G. Velárde
·
YOU?
·
· 2016
· Open Access
·
· DOI: https://doi.org/10.3390/e18030092
YOU?
·
· 2016
· Open Access
·
· DOI: https://doi.org/10.3390/e18030092
We study here several simple models of the electron transfer (ET) in a one-dimensional nonlinear lattice between a donor and an acceptor and propose a new fast mechanism of electron surfing on soliton-like excitations along the lattice. The nonlinear lattice is modeled as a classical one-dimensional Morse chain and the dynamics of the electrons are considered in the tight-binding approximation. This model is applied to the processes along a covalent bridge connecting donors and acceptors. First, it is shown that the electron forms bound states with the solitonic excitations in the lattice. These so-called solectrons may move with supersonic speed. In a heated system, the electron transfer between a donor and an acceptor is modeled as a diffusion-like process. We study in detail the role of thermal factors on the electron transfer. Then, we develop a simple model based on the classical Smoluchowski–Chandrasekhar picture of diffusion-controlled reactions as stochastic processes with emitters and absorbers. Acceptors are modeled by an absorbing boundary. Finally, we compare the new ET mechanisms described here with known ET data. We conclude that electron surfing on solitons could be a special fast way for ET over quite long distances.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/e18030092
- https://www.mdpi.com/1099-4300/18/3/92/pdf?version=1457704435
- OA Status
- gold
- Cited By
- 7
- References
- 52
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2295845335
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Raw OpenAlex JSON
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https://openalex.org/W2295845335Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/e18030092Digital Object Identifier
- Title
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Long-Range Electron Transport Donor-Acceptor in Nonlinear LatticesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2016Year of publication
- Publication date
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2016-03-11Full publication date if available
- Authors
-
A. P. Chetverikov, W. Ebeling, Manuel G. VelárdeList of authors in order
- Landing page
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https://doi.org/10.3390/e18030092Publisher landing page
- PDF URL
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https://www.mdpi.com/1099-4300/18/3/92/pdf?version=1457704435Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://www.mdpi.com/1099-4300/18/3/92/pdf?version=1457704435Direct OA link when available
- Concepts
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Electron, Lattice (music), Physics, Electron transfer, Nonlinear system, Acceptor, Statistical physics, Molecular physics, Quantum mechanics, Chemical physics, Atomic physics, Chemistry, Physical chemistry, AcousticsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
7Total citation count in OpenAlex
- Citations by year (recent)
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2024: 1, 2023: 1, 2022: 1, 2019: 1, 2017: 3Per-year citation counts (last 5 years)
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52Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| primary_location.raw_source_name | Entropy |
| primary_location.landing_page_url | https://doi.org/10.3390/e18030092 |
| publication_date | 2016-03-11 |
| publication_year | 2016 |
| referenced_works | https://openalex.org/W51419519, https://openalex.org/W1984545350, https://openalex.org/W1967609487, https://openalex.org/W2093041725, https://openalex.org/W2023693337, https://openalex.org/W2026128357, https://openalex.org/W2091201245, https://openalex.org/W1985793583, https://openalex.org/W1978559032, https://openalex.org/W2160066452, https://openalex.org/W2144462742, https://openalex.org/W1954706274, https://openalex.org/W3102272679, https://openalex.org/W2031904472, https://openalex.org/W2044990980, https://openalex.org/W2105348198, https://openalex.org/W2085541270, https://openalex.org/W2094025206, https://openalex.org/W2105884320, https://openalex.org/W2135557059, https://openalex.org/W2156859795, https://openalex.org/W2166090671, https://openalex.org/W2006121157, https://openalex.org/W2059295184, https://openalex.org/W2019297732, https://openalex.org/W2134566140, https://openalex.org/W2132614221, https://openalex.org/W2129837914, https://openalex.org/W4298029373, https://openalex.org/W2088560539, https://openalex.org/W2011904285, https://openalex.org/W2073565275, https://openalex.org/W4254320933, https://openalex.org/W2031527250, https://openalex.org/W2116726628, https://openalex.org/W3141350321, https://openalex.org/W2032805951, https://openalex.org/W2009101818, https://openalex.org/W1967090528, https://openalex.org/W1989643187, https://openalex.org/W2147418907, https://openalex.org/W2162488624, https://openalex.org/W1516991785, https://openalex.org/W2053167395, https://openalex.org/W1989263327, https://openalex.org/W2079715570, https://openalex.org/W4247930035, https://openalex.org/W2054610454, https://openalex.org/W656139762, https://openalex.org/W127786, https://openalex.org/W640502517, https://openalex.org/W2167879962 |
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| corresponding_author_ids | https://openalex.org/A5087999746 |
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| corresponding_institution_ids | https://openalex.org/I121748325 |
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