Low-Temperature Synthesis of Highly Efficient, Deep-Red Zn-Cu-In-Se/ZnSe Fluorescence Quantum Dots Article Swipe
Juan Yang
,
Jingling Li
,
Yanqing Zhu
,
Xueqing Xu
,
Xiudi Xiao
,
Bing Deng
,
Kaili Qin
,
Zhuoneng Bi
,
Shuaijun Chen
,
Gang Xu
·
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.1142/s179329201950070x
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.1142/s179329201950070x
We report a facile synthesis method on CuInSe 2 (CISe)-based quantum dots (QDs) by using tri-[Formula: see text]-octylphosphine selenium (TOPSe) as selenide precursor, with assistance of oleylamine (OAm) and [Formula: see text]-dodecanethiol (DDT). We demonstrate that the OAm and DDT jointly contribute to the formation of the low-temperature-decomposable metal-sulfide clusters, and promote the QD nucleation at relatively low temperature range of 180–200 ∘ C. Furthermore, to improve fluorescence property, Zn-doping and ZnSe coating are simultaneously carried out. The obtained deep-red ZnCISe/ZnSe QDs possess higher quantum yield of 65% at wavelength of 670[Formula: see text]nm, which is in the best performance range ever reported. Then, we investigate the improvement mechanism, where the sufficient Zn replacement of In sites is the crucial factor. This modified core–shell structure provides two benefits, on the one hand, the enhancement on intrinsic defect-related recombination, and the other hand, the improved core–shell interface that reduces the nonradiative recombination.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1142/s179329201950070x
- https://www.worldscientific.com/doi/pdf/10.1142/S179329201950070X
- OA Status
- bronze
- Cited By
- 2
- References
- 28
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2942741861
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- OpenAlex ID
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https://openalex.org/W2942741861Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1142/s179329201950070xDigital Object Identifier
- Title
-
Low-Temperature Synthesis of Highly Efficient, Deep-Red Zn-Cu-In-Se/ZnSe Fluorescence Quantum DotsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2019Year of publication
- Publication date
-
2019-05-03Full publication date if available
- Authors
-
Juan Yang, Jingling Li, Yanqing Zhu, Xueqing Xu, Xiudi Xiao, Bing Deng, Kaili Qin, Zhuoneng Bi, Shuaijun Chen, Gang XuList of authors in order
- Landing page
-
https://doi.org/10.1142/s179329201950070xPublisher landing page
- PDF URL
-
https://www.worldscientific.com/doi/pdf/10.1142/S179329201950070XDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
bronzeOpen access status per OpenAlex
- OA URL
-
https://www.worldscientific.com/doi/pdf/10.1142/S179329201950070XDirect OA link when available
- Concepts
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Oleylamine, Quantum dot, Quantum yield, Materials science, Nucleation, Fluorescence, Selenide, Core (optical fiber), Yield (engineering), Cadmium sulfide, Range (aeronautics), Optoelectronics, Nanocrystal, Nanotechnology, Selenium, Optics, Chemistry, Physics, Composite material, Metallurgy, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 1, 2020: 1Per-year citation counts (last 5 years)
- References (count)
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28Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.OAm | 37 |
| abstract_inverted_index.QDs | 81 |
| abstract_inverted_index.The | 77 |
| abstract_inverted_index.and | 28, 38, 50, 70, 138 |
| abstract_inverted_index.are | 73 |
| abstract_inverted_index.low | 57 |
| abstract_inverted_index.one | 130 |
| abstract_inverted_index.see | 16, 30, 92 |
| abstract_inverted_index.the | 36, 43, 46, 52, 97, 106, 110, 118, 129, 132, 139, 142, 148 |
| abstract_inverted_index.two | 126 |
| abstract_inverted_index.∘ | 62 |
| abstract_inverted_index.This | 121 |
| abstract_inverted_index.ZnSe | 71 |
| abstract_inverted_index.best | 98 |
| abstract_inverted_index.dots | 11 |
| abstract_inverted_index.ever | 101 |
| abstract_inverted_index.out. | 76 |
| abstract_inverted_index.that | 35, 146 |
| abstract_inverted_index.with | 23 |
| abstract_inverted_index.(OAm) | 27 |
| abstract_inverted_index.(QDs) | 12 |
| abstract_inverted_index.Then, | 103 |
| abstract_inverted_index.hand, | 131, 141 |
| abstract_inverted_index.other | 140 |
| abstract_inverted_index.range | 59, 100 |
| abstract_inverted_index.sites | 116 |
| abstract_inverted_index.using | 14 |
| abstract_inverted_index.where | 109 |
| abstract_inverted_index.which | 94 |
| abstract_inverted_index.yield | 85 |
| abstract_inverted_index.(DDT). | 32 |
| abstract_inverted_index.CuInSe | 7 |
| abstract_inverted_index.facile | 3 |
| abstract_inverted_index.higher | 83 |
| abstract_inverted_index.method | 5 |
| abstract_inverted_index.report | 1 |
| abstract_inverted_index.(TOPSe) | 19 |
| abstract_inverted_index.carried | 75 |
| abstract_inverted_index.coating | 72 |
| abstract_inverted_index.crucial | 119 |
| abstract_inverted_index.factor. | 120 |
| abstract_inverted_index.improve | 66 |
| abstract_inverted_index.jointly | 40 |
| abstract_inverted_index.possess | 82 |
| abstract_inverted_index.promote | 51 |
| abstract_inverted_index.quantum | 10, 84 |
| abstract_inverted_index.reduces | 147 |
| abstract_inverted_index.deep-red | 79 |
| abstract_inverted_index.improved | 143 |
| abstract_inverted_index.modified | 122 |
| abstract_inverted_index.obtained | 78 |
| abstract_inverted_index.provides | 125 |
| abstract_inverted_index.selenide | 21 |
| abstract_inverted_index.selenium | 18 |
| abstract_inverted_index.text]nm, | 93 |
| abstract_inverted_index.180–200 | 61 |
| abstract_inverted_index.Zn-doping | 69 |
| abstract_inverted_index.[Formula: | 29 |
| abstract_inverted_index.benefits, | 127 |
| abstract_inverted_index.clusters, | 49 |
| abstract_inverted_index.formation | 44 |
| abstract_inverted_index.interface | 145 |
| abstract_inverted_index.intrinsic | 135 |
| abstract_inverted_index.property, | 68 |
| abstract_inverted_index.reported. | 102 |
| abstract_inverted_index.structure | 124 |
| abstract_inverted_index.synthesis | 4 |
| abstract_inverted_index.assistance | 24 |
| abstract_inverted_index.contribute | 41 |
| abstract_inverted_index.mechanism, | 108 |
| abstract_inverted_index.nucleation | 54 |
| abstract_inverted_index.oleylamine | 26 |
| abstract_inverted_index.precursor, | 22 |
| abstract_inverted_index.relatively | 56 |
| abstract_inverted_index.sufficient | 111 |
| abstract_inverted_index.wavelength | 89 |
| abstract_inverted_index.ZnCISe/ZnSe | 80 |
| abstract_inverted_index.demonstrate | 34 |
| abstract_inverted_index.enhancement | 133 |
| abstract_inverted_index.improvement | 107 |
| abstract_inverted_index.investigate | 105 |
| abstract_inverted_index.performance | 99 |
| abstract_inverted_index.replacement | 113 |
| abstract_inverted_index.temperature | 58 |
| abstract_inverted_index.(CISe)-based | 9 |
| abstract_inverted_index.670[Formula: | 91 |
| abstract_inverted_index.Furthermore, | 64 |
| abstract_inverted_index.core–shell | 123, 144 |
| abstract_inverted_index.fluorescence | 67 |
| abstract_inverted_index.nonradiative | 149 |
| abstract_inverted_index.metal-sulfide | 48 |
| abstract_inverted_index.tri-[Formula: | 15 |
| abstract_inverted_index.defect-related | 136 |
| abstract_inverted_index.recombination, | 137 |
| abstract_inverted_index.recombination. | 150 |
| abstract_inverted_index.simultaneously | 74 |
| abstract_inverted_index.text]-dodecanethiol | 31 |
| abstract_inverted_index.text]-octylphosphine | 17 |
| abstract_inverted_index.low-temperature-decomposable | 47 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 89 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 10 |
| citation_normalized_percentile.value | 0.36723895 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |