Low‐Energy, Ultrafast Spin Reorientation at Competing Hybrid Interfaces with Tunable Operating Temperature Article Swipe
YOU?
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· 2025
· Open Access
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· DOI: https://doi.org/10.1002/adma.202419192
Information can be stored in magnetic materials by encoding with the direction of the magnetic moment. A figure of merit for these systems is the energy needed to rewrite the information by changing the magnetic moment. Organic molecules offer a playground to manipulate spin order, with metallo‐molecular interfaces being a promising direction for sustainable devices. Here, a spin reorientation transition is demonstrated in molecular interfaces of 3d ferromagnetic films due to a competition between a perpendicular magnetic anisotropy (PMA) induced by a heavy metal that dominates at high temperatures, and an in‐plane anisotropy generated by molecular coupling at low temperatures. The transition can be tuned around room temperature by varying the ferromagnet thickness (1.4 – 1.9 nm) or the choice of molecular overlayer, with the organic molecules being C 60 , hydrogen, and metal (Cu, Co) phthalocyanines. Near the transition temperature, the magnetisation easy axis can be switched with a small energy input, either electrically with a current density of 10 5 A cm −2 , or optically by a fs laser pulse of fluence as low as 0.12 mJ cm −2 , suggesting heat assisted technology applications. Magnetic dichroism measurements point toward a phase transition at the organic interface being responsible for the spin reorientation transition.
Related Topics
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202419192
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202419192
- OA Status
- hybrid
- References
- 52
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4412956057
Raw OpenAlex JSON
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https://openalex.org/W4412956057Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202419192Digital Object Identifier
- Title
-
Low‐Energy, Ultrafast Spin Reorientation at Competing Hybrid Interfaces with Tunable Operating TemperatureWork title
- Type
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articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2025Year of publication
- Publication date
-
2025-08-05Full publication date if available
- Authors
-
Servet Ozdemir, Matthew Rogers, J. Strohsack, V. Hari Babu, Manuel Valvidares, Thahabh Haddadi, Parvathy Harikumar, David D. O’Regan, Gilberto Teobaldi, Timothy Moorsom, M. Ali, Gavin Burnell, B. J. Hickey, T. Mertelj, Oscar CéspedesList of authors in order
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https://doi.org/10.1002/adma.202419192Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202419192Direct link to full text PDF
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202419192Direct OA link when available
- Concepts
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Materials science, Condensed matter physics, Overlayer, Magnetization, Ferromagnetism, Magnetic anisotropy, Anisotropy energy, Magnetic moment, Spin (aerodynamics), Chemical physics, Magnetic field, Chemistry, Aerospace engineering, Physics, Engineering, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
- References (count)
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52Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.−2 | 165, 182 |
| abstract_inverted_index.(PMA) | 79 |
| abstract_inverted_index.Here, | 56 |
| abstract_inverted_index.being | 49, 128, 201 |
| abstract_inverted_index.films | 69 |
| abstract_inverted_index.heavy | 83 |
| abstract_inverted_index.laser | 172 |
| abstract_inverted_index.merit | 20 |
| abstract_inverted_index.metal | 84, 134 |
| abstract_inverted_index.offer | 39 |
| abstract_inverted_index.phase | 195 |
| abstract_inverted_index.point | 192 |
| abstract_inverted_index.pulse | 173 |
| abstract_inverted_index.small | 151 |
| abstract_inverted_index.these | 22 |
| abstract_inverted_index.tuned | 105 |
| abstract_inverted_index.around | 106 |
| abstract_inverted_index.choice | 120 |
| abstract_inverted_index.either | 154 |
| abstract_inverted_index.energy | 26, 152 |
| abstract_inverted_index.figure | 18 |
| abstract_inverted_index.input, | 153 |
| abstract_inverted_index.needed | 27 |
| abstract_inverted_index.order, | 45 |
| abstract_inverted_index.stored | 4 |
| abstract_inverted_index.toward | 193 |
| abstract_inverted_index.Organic | 37 |
| abstract_inverted_index.between | 74 |
| abstract_inverted_index.current | 158 |
| abstract_inverted_index.density | 159 |
| abstract_inverted_index.fluence | 175 |
| abstract_inverted_index.induced | 80 |
| abstract_inverted_index.moment. | 16, 36 |
| abstract_inverted_index.organic | 126, 199 |
| abstract_inverted_index.rewrite | 29 |
| abstract_inverted_index.systems | 23 |
| abstract_inverted_index.varying | 110 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.Magnetic | 189 |
| abstract_inverted_index.assisted | 186 |
| abstract_inverted_index.changing | 33 |
| abstract_inverted_index.coupling | 97 |
| abstract_inverted_index.devices. | 55 |
| abstract_inverted_index.encoding | 9 |
| abstract_inverted_index.magnetic | 6, 15, 35, 77 |
| abstract_inverted_index.switched | 148 |
| abstract_inverted_index.dichroism | 190 |
| abstract_inverted_index.direction | 12, 52 |
| abstract_inverted_index.dominates | 86 |
| abstract_inverted_index.generated | 94 |
| abstract_inverted_index.hydrogen, | 132 |
| abstract_inverted_index.interface | 200 |
| abstract_inverted_index.materials | 7 |
| abstract_inverted_index.molecular | 64, 96, 122 |
| abstract_inverted_index.molecules | 38, 127 |
| abstract_inverted_index.optically | 168 |
| abstract_inverted_index.promising | 51 |
| abstract_inverted_index.thickness | 113 |
| abstract_inverted_index.anisotropy | 78, 93 |
| abstract_inverted_index.interfaces | 48, 65 |
| abstract_inverted_index.in‐plane | 92 |
| abstract_inverted_index.manipulate | 43 |
| abstract_inverted_index.overlayer, | 123 |
| abstract_inverted_index.playground | 41 |
| abstract_inverted_index.suggesting | 184 |
| abstract_inverted_index.technology | 187 |
| abstract_inverted_index.transition | 60, 102, 140, 196 |
| abstract_inverted_index.Information | 1 |
| abstract_inverted_index.competition | 73 |
| abstract_inverted_index.ferromagnet | 112 |
| abstract_inverted_index.information | 31 |
| abstract_inverted_index.responsible | 202 |
| abstract_inverted_index.sustainable | 54 |
| abstract_inverted_index.temperature | 108 |
| abstract_inverted_index.transition. | 207 |
| abstract_inverted_index.demonstrated | 62 |
| abstract_inverted_index.electrically | 155 |
| abstract_inverted_index.measurements | 191 |
| abstract_inverted_index.temperature, | 141 |
| abstract_inverted_index.applications. | 188 |
| abstract_inverted_index.ferromagnetic | 68 |
| abstract_inverted_index.magnetisation | 143 |
| abstract_inverted_index.perpendicular | 76 |
| abstract_inverted_index.reorientation | 59, 206 |
| abstract_inverted_index.temperatures, | 89 |
| abstract_inverted_index.temperatures. | 100 |
| abstract_inverted_index.phthalocyanines. | 137 |
| abstract_inverted_index.metallo‐molecular | 47 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5012415319, https://openalex.org/A5006928498 |
| countries_distinct_count | 4 |
| institutions_distinct_count | 15 |
| corresponding_institution_ids | https://openalex.org/I130828816 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/12 |
| sustainable_development_goals[0].score | 0.41999998688697815 |
| sustainable_development_goals[0].display_name | Responsible consumption and production |
| citation_normalized_percentile.value | 0.274275 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |