Luminescence and Structural Characterization of Gd2O2S Scintillators Doped with Tb3+, Ce3+, Pr3+ and F for Imaging Applications Article Swipe
Alessia De Martinis
,
Luigi Montalto
,
Lorenzo Scalise
,
D. Rinaldi
,
P. Mengucci
,
C. Michail
,
George Fountos
,
Nicki Martini
,
V. Koukou
,
Ioannis Valais
,
Athanasios Bakas
,
Christina Fountzoula
,
I. Kandarakis
,
S. David
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/cryst12060854
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/cryst12060854
Radiodiagnostic technologies are powerful tools for preventing diseases and monitoring the condition of patients. Medicine and sectors such as industry and research all use this inspection methodology. This field demands innovative and more sophisticated systems and materials for improving resolution and sensitivity, leading to a faster, reliable, and safe diagnosis. In this study, a large characterization of gadolinium oxysulfide (Gd2O2S) scintillator screens for imaging applications has been carried out. Seven scintillator samples were doped with praseodymium (Pr3+), terbium (Tb3+) activators and co-doped with praseodymium, cerium, and fluorine (Gd2O2S:Pr,Ce,F). The sample screens were prepared in the laboratory in the form of high packing density screens, following the methodology used in screen sample preparation in infrared spectroscopy and luminescence. Parameters such as quantum detection efficiency (QDE), energy absorption efficiency (EAE), and absolute luminescence efficiency (ALE) were evaluated. In parallel, a structural characterization was performed, via XRD and SEM analysis, for quality control purposes as well as for correlation with optical properties. Spatial resolution properties were experimentally evaluated via the Modulation Transfer Function. Results were compared with published data about Gd2O2S:Pr,Ce,F screens produced with a standard method of a sedimentation technique. In particular, the ALE rose with the X-ray tube voltage up to 100 kVp, while among the different dopants, Gd2O2S:Pr exhibited the highest ALE value. When comparing screens with different thicknesses, a linear trend for the ALE value was not observed; the highest ALE value was measured for the 0.57 mm thick Gd2O2S:Pr,Ce,F sample, while the best MTF values were found in the thinner Gd2O2S:Pr,Ce,F screen with 0.38 mm thickness.
Related Topics
Concepts
Praseodymium
Scintillator
Luminescence
Materials science
Effective atomic number
Terbium
Doping
Dopant
Characterization (materials science)
Gadolinium
Cerium
Optical transfer function
Analytical Chemistry (journal)
Optics
Optoelectronics
Nanotechnology
Chemistry
Physics
Photon
Chromatography
Metallurgy
Detector
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/cryst12060854
- https://www.mdpi.com/2073-4352/12/6/854/pdf?version=1655710121
- OA Status
- gold
- Cited By
- 12
- References
- 33
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4283025892
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4283025892Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3390/cryst12060854Digital Object Identifier
- Title
-
Luminescence and Structural Characterization of Gd2O2S Scintillators Doped with Tb3+, Ce3+, Pr3+ and F for Imaging ApplicationsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-06-17Full publication date if available
- Authors
-
Alessia De Martinis, Luigi Montalto, Lorenzo Scalise, D. Rinaldi, P. Mengucci, C. Michail, George Fountos, Nicki Martini, V. Koukou, Ioannis Valais, Athanasios Bakas, Christina Fountzoula, I. Kandarakis, S. DavidList of authors in order
- Landing page
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https://doi.org/10.3390/cryst12060854Publisher landing page
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https://www.mdpi.com/2073-4352/12/6/854/pdf?version=1655710121Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://www.mdpi.com/2073-4352/12/6/854/pdf?version=1655710121Direct OA link when available
- Concepts
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Praseodymium, Scintillator, Luminescence, Materials science, Effective atomic number, Terbium, Doping, Dopant, Characterization (materials science), Gadolinium, Cerium, Optical transfer function, Analytical Chemistry (journal), Optics, Optoelectronics, Nanotechnology, Chemistry, Physics, Photon, Chromatography, Metallurgy, DetectorTop concepts (fields/topics) attached by OpenAlex
- Cited by
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12Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2, 2024: 9, 2023: 1Per-year citation counts (last 5 years)
- References (count)
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33Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.and | 8, 15, 20, 31, 35, 40, 47, 80, 85, 115, 128, 144 |
| abstract_inverted_index.are | 2 |
| abstract_inverted_index.for | 5, 37, 62, 147, 154, 222, 235 |
| abstract_inverted_index.has | 65 |
| abstract_inverted_index.not | 227 |
| abstract_inverted_index.the | 10, 94, 97, 105, 166, 190, 194, 204, 209, 223, 229, 236, 243, 250 |
| abstract_inverted_index.use | 23 |
| abstract_inverted_index.via | 142, 165 |
| abstract_inverted_index.was | 140, 226, 233 |
| abstract_inverted_index.0.38 | 255 |
| abstract_inverted_index.0.57 | 237 |
| abstract_inverted_index.This | 27 |
| abstract_inverted_index.When | 213 |
| abstract_inverted_index.been | 66 |
| abstract_inverted_index.best | 244 |
| abstract_inverted_index.data | 175 |
| abstract_inverted_index.form | 98 |
| abstract_inverted_index.high | 100 |
| abstract_inverted_index.kVp, | 201 |
| abstract_inverted_index.more | 32 |
| abstract_inverted_index.out. | 68 |
| abstract_inverted_index.rose | 192 |
| abstract_inverted_index.safe | 48 |
| abstract_inverted_index.such | 17, 118 |
| abstract_inverted_index.this | 24, 51 |
| abstract_inverted_index.tube | 196 |
| abstract_inverted_index.used | 107 |
| abstract_inverted_index.well | 152 |
| abstract_inverted_index.were | 72, 91, 133, 162, 171, 247 |
| abstract_inverted_index.with | 74, 82, 156, 173, 180, 193, 216, 254 |
| abstract_inverted_index.(ALE) | 132 |
| abstract_inverted_index.Seven | 69 |
| abstract_inverted_index.X-ray | 195 |
| abstract_inverted_index.about | 176 |
| abstract_inverted_index.among | 203 |
| abstract_inverted_index.doped | 73 |
| abstract_inverted_index.field | 28 |
| abstract_inverted_index.found | 248 |
| abstract_inverted_index.large | 54 |
| abstract_inverted_index.thick | 239 |
| abstract_inverted_index.tools | 4 |
| abstract_inverted_index.trend | 221 |
| abstract_inverted_index.value | 225, 232 |
| abstract_inverted_index.while | 202, 242 |
| abstract_inverted_index.(EAE), | 127 |
| abstract_inverted_index.(QDE), | 123 |
| abstract_inverted_index.(Tb3+) | 78 |
| abstract_inverted_index.energy | 124 |
| abstract_inverted_index.linear | 220 |
| abstract_inverted_index.method | 183 |
| abstract_inverted_index.sample | 89, 110 |
| abstract_inverted_index.screen | 109, 253 |
| abstract_inverted_index.study, | 52 |
| abstract_inverted_index.value. | 212 |
| abstract_inverted_index.values | 246 |
| abstract_inverted_index.(Pr3+), | 76 |
| abstract_inverted_index.Results | 170 |
| abstract_inverted_index.Spatial | 159 |
| abstract_inverted_index.carried | 67 |
| abstract_inverted_index.cerium, | 84 |
| abstract_inverted_index.control | 149 |
| abstract_inverted_index.demands | 29 |
| abstract_inverted_index.density | 102 |
| abstract_inverted_index.faster, | 45 |
| abstract_inverted_index.highest | 210, 230 |
| abstract_inverted_index.imaging | 63 |
| abstract_inverted_index.leading | 42 |
| abstract_inverted_index.optical | 157 |
| abstract_inverted_index.packing | 101 |
| abstract_inverted_index.quality | 148 |
| abstract_inverted_index.quantum | 120 |
| abstract_inverted_index.sample, | 241 |
| abstract_inverted_index.samples | 71 |
| abstract_inverted_index.screens | 61, 90, 178, 215 |
| abstract_inverted_index.sectors | 16 |
| abstract_inverted_index.systems | 34 |
| abstract_inverted_index.terbium | 77 |
| abstract_inverted_index.thinner | 251 |
| abstract_inverted_index.voltage | 197 |
| abstract_inverted_index.(Gd2O2S) | 59 |
| abstract_inverted_index.Medicine | 14 |
| abstract_inverted_index.Transfer | 168 |
| abstract_inverted_index.absolute | 129 |
| abstract_inverted_index.co-doped | 81 |
| abstract_inverted_index.compared | 172 |
| abstract_inverted_index.diseases | 7 |
| abstract_inverted_index.dopants, | 206 |
| abstract_inverted_index.fluorine | 86 |
| abstract_inverted_index.industry | 19 |
| abstract_inverted_index.infrared | 113 |
| abstract_inverted_index.measured | 234 |
| abstract_inverted_index.powerful | 3 |
| abstract_inverted_index.prepared | 92 |
| abstract_inverted_index.produced | 179 |
| abstract_inverted_index.purposes | 150 |
| abstract_inverted_index.research | 21 |
| abstract_inverted_index.screens, | 103 |
| abstract_inverted_index.standard | 182 |
| abstract_inverted_index.Function. | 169 |
| abstract_inverted_index.Gd2O2S:Pr | 207 |
| abstract_inverted_index.analysis, | 146 |
| abstract_inverted_index.comparing | 214 |
| abstract_inverted_index.condition | 11 |
| abstract_inverted_index.detection | 121 |
| abstract_inverted_index.different | 205, 217 |
| abstract_inverted_index.evaluated | 164 |
| abstract_inverted_index.exhibited | 208 |
| abstract_inverted_index.following | 104 |
| abstract_inverted_index.improving | 38 |
| abstract_inverted_index.materials | 36 |
| abstract_inverted_index.observed; | 228 |
| abstract_inverted_index.parallel, | 136 |
| abstract_inverted_index.patients. | 13 |
| abstract_inverted_index.published | 174 |
| abstract_inverted_index.reliable, | 46 |
| abstract_inverted_index.Modulation | 167 |
| abstract_inverted_index.Parameters | 117 |
| abstract_inverted_index.absorption | 125 |
| abstract_inverted_index.activators | 79 |
| abstract_inverted_index.diagnosis. | 49 |
| abstract_inverted_index.efficiency | 122, 126, 131 |
| abstract_inverted_index.evaluated. | 134 |
| abstract_inverted_index.gadolinium | 57 |
| abstract_inverted_index.innovative | 30 |
| abstract_inverted_index.inspection | 25 |
| abstract_inverted_index.laboratory | 95 |
| abstract_inverted_index.monitoring | 9 |
| abstract_inverted_index.oxysulfide | 58 |
| abstract_inverted_index.performed, | 141 |
| abstract_inverted_index.preventing | 6 |
| abstract_inverted_index.properties | 161 |
| abstract_inverted_index.resolution | 39, 160 |
| abstract_inverted_index.structural | 138 |
| abstract_inverted_index.technique. | 187 |
| abstract_inverted_index.thickness. | 257 |
| abstract_inverted_index.correlation | 155 |
| abstract_inverted_index.methodology | 106 |
| abstract_inverted_index.particular, | 189 |
| abstract_inverted_index.preparation | 111 |
| abstract_inverted_index.properties. | 158 |
| abstract_inverted_index.applications | 64 |
| abstract_inverted_index.luminescence | 130 |
| abstract_inverted_index.methodology. | 26 |
| abstract_inverted_index.praseodymium | 75 |
| abstract_inverted_index.scintillator | 60, 70 |
| abstract_inverted_index.sensitivity, | 41 |
| abstract_inverted_index.spectroscopy | 114 |
| abstract_inverted_index.technologies | 1 |
| abstract_inverted_index.thicknesses, | 218 |
| abstract_inverted_index.luminescence. | 116 |
| abstract_inverted_index.praseodymium, | 83 |
| abstract_inverted_index.sedimentation | 186 |
| abstract_inverted_index.sophisticated | 33 |
| abstract_inverted_index.Gd2O2S:Pr,Ce,F | 177, 240, 252 |
| abstract_inverted_index.experimentally | 163 |
| abstract_inverted_index.Radiodiagnostic | 0 |
| abstract_inverted_index.characterization | 55, 139 |
| abstract_inverted_index.(Gd2O2S:Pr,Ce,F). | 87 |
| cited_by_percentile_year.max | 99 |
| cited_by_percentile_year.min | 89 |
| corresponding_author_ids | https://openalex.org/A5038884754 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 14 |
| corresponding_institution_ids | https://openalex.org/I122534668 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.8100000023841858 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile.value | 0.91929702 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |