Luminescence Properties of Al₂O₃:Ti in the Blue and Red Regions: A Combined Theoretical and Experimental Study Article Swipe

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Théo Cavignac , Maxence Vigier , Emmanuel Fritsch , Philippe Deniard , Stéphane Jobic , Camille Latouche ·

YOU? · · 2024 · Open Access · · DOI: https://doi.org/10.1021/acs.inorgchem.3c03476

Using jointly experimental results and first-principles calculations, we unambiguously assign the underlying mechanisms behind two commonly observed luminescence bands for the Al₂O₃ material. Indeed, we show that the red band is associated with a Ti³⁺ d-d transition as expected, while the blue band is the combination of the Ti³⁺ + O^- → Ti⁴⁺ + O^2- and V_O^•+e^- → V_O^× de-excitation processes. Thanks to our recent developments, which take into account the vibrational contributions to the electronic transitions in solids, we were able to simulate the luminescence spectra for the different signatures. The excellent agreement with the experiment demonstrates that it should be possible to predict the color of the material with a CIE chromaticity diagram. We also anticipated the luminescence signature of Al₂O₃:Ti,Ca and Al₂O₃:Ti,Be that were confirmed by experiment.

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Luminescence

Chromaticity

Chemistry

Excitation (Magnetic)

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Luminescence Chromaticity Chemistry Excitation Persistent luminescence Diagram Atomic electron transition Spectral line Molecular physics Analytical Chemistry (journal) Atomic physics Chemical physics Optics Physics Chromatography Quantum mechanics Mathematics Astronomy Thermoluminescence Statistics

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Type: article
Language: en
Landing Page: https://doi.org/10.1021/acs.inorgchem.3c03476
OA Status: green
Cited By: 3
References: 82
Related Works: 10
OpenAlex ID: https://openalex.org/W4391485161

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DOI: https://doi.org/10.1021/acs.inorgchem.3c03476

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Title: Luminescence Properties of Al₂O₃:Ti in the Blue and Red Regions: A Combined Theoretical and Experimental Study

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Language: en

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Publication year: 2024

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Publication date: 2024-02-02

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Authors: Théo Cavignac, Maxence Vigier, Emmanuel Fritsch, Philippe Deniard, Stéphane Jobic, Camille Latouche

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Landing page: https://doi.org/10.1021/acs.inorgchem.3c03476

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Concepts: Luminescence, Chromaticity, Chemistry, Excitation, Persistent luminescence, Diagram, Atomic electron transition, Spectral line, Molecular physics, Analytical Chemistry (journal), Atomic physics, Chemical physics, Optics, Physics, Chromatography, Quantum mechanics, Mathematics, Astronomy, Thermoluminescence, Statistics

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Cited by: 3

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Luminescence Properties of Al2O3:Ti in the Blue and Red Regions: A Combined Theoretical and Experimental Study Article Swipe

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Luminescence Properties of Al₂O₃:Ti in the Blue and Red Regions: A Combined Theoretical and Experimental Study Article Swipe