Magnetically and optically active edges in phosphorene nanoribbons Article Swipe
Arjun Ashoka
,
Adam J. Clancy
,
Naitik A. Panjwani
,
Adam L. Cronin
,
Loren Picco
,
Eva S. Y. Aw
,
Nicholas J. M. Popiel
,
Alexander G. Eaton
,
Thomas G. Parton
,
Rebecca R. C. Shutt
,
Sascha Feldmann
,
Remington Carey
,
Thomas J. Macdonald
,
Cheng Liu
,
Marion E. Severijnen
,
Sandra Kleuskens
,
Loreta A. Muscarella
,
Felix R. Fischer
,
Hilton B. de Aguiar
,
Richard H. Friend
,
Jan Behrends
,
Peter C. M. Christianen
,
Christopher A. Howard
,
Raj Pandya
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41586-024-08563-x
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41586-024-08563-x
Nanoribbons, nanometre-wide strips of a two-dimensional material, are a unique system in condensed matter. They combine the exotic electronic structures of low-dimensional materials with an enhanced number of exposed edges, where phenomena including ultralong spin coherence times 1,2 , quantum confinement 3 and topologically protected states 4,5 can emerge. An exciting prospect for this material concept is the potential for both a tunable semiconducting electronic structure and magnetism along the nanoribbon edge, a key property for spin-based electronics such as (low-energy) non-volatile transistors 6 . Here we report the magnetic and semiconducting properties of phosphorene nanoribbons (PNRs). We demonstrate that at room temperature, films of PNRs show macroscopic magnetic properties arising from their edge, with internal fields of roughly 240 to 850 mT. In solution, a giant magnetic anisotropy enables the alignment of PNRs at sub-1-T fields. By leveraging this alignment effect, we discover that on photoexcitation, energy is rapidly funnelled to a state that is localized to the magnetic edge and coupled to a symmetry-forbidden edge phonon mode. Our results establish PNRs as a fascinating system for studying the interplay between magnetism and semiconducting ground states at room temperature and provide a stepping-stone towards using low-dimensional nanomaterials in quantum electronics.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41586-024-08563-x
- https://www.nature.com/articles/s41586-024-08563-x.pdf
- OA Status
- hybrid
- Cited By
- 6
- References
- 63
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4408357297
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4408357297Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41586-024-08563-xDigital Object Identifier
- Title
-
Magnetically and optically active edges in phosphorene nanoribbonsWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2025Year of publication
- Publication date
-
2025-03-12Full publication date if available
- Authors
-
Arjun Ashoka, Adam J. Clancy, Naitik A. Panjwani, Adam L. Cronin, Loren Picco, Eva S. Y. Aw, Nicholas J. M. Popiel, Alexander G. Eaton, Thomas G. Parton, Rebecca R. C. Shutt, Sascha Feldmann, Remington Carey, Thomas J. Macdonald, Cheng Liu, Marion E. Severijnen, Sandra Kleuskens, Loreta A. Muscarella, Felix R. Fischer, Hilton B. de Aguiar, Richard H. Friend, Jan Behrends, Peter C. M. Christianen, Christopher A. Howard, Raj PandyaList of authors in order
- Landing page
-
https://doi.org/10.1038/s41586-024-08563-xPublisher landing page
- PDF URL
-
https://www.nature.com/articles/s41586-024-08563-x.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
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https://www.nature.com/articles/s41586-024-08563-x.pdfDirect OA link when available
- Concepts
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Phosphorene, Magnetism, Condensed matter physics, Materials science, Spintronics, Photoexcitation, Nanomaterials, Spin (aerodynamics), Nanotechnology, Physics, Ferromagnetism, Monolayer, Excited state, Thermodynamics, Nuclear physicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
6Total citation count in OpenAlex
- Citations by year (recent)
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2025: 6Per-year citation counts (last 5 years)
- References (count)
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63Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| citation_normalized_percentile.value | 0.95894744 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |