Manipulating electronic band of NiO/NiMoO4–x nanosheets as robust bifunctional catalyst for water splitting Article Swipe
Qiyu Liu
,
Jintao Zhang
,
Jingwen He
,
Peng Zhang
,
Zujin Yang
,
Xihong Lu
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.nxnano.2025.100173
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.nxnano.2025.100173
Due to the issues of energy shortage and environmental pollution, it is crucial to explore environmentally friendly and efficient bifunctional catalysts for oxygen and hydrogen evolution reaction (OER/HER). Herein, we demonstrate an oxygen vacancy-rich NiO/NiMoO4 heterojunction as bifunctional catalyst for electrocatalytic water splitting (denoted as NiO/NiMoO4–x) on commercial nickel foam by a facile hydrothermal-calcination method. The experimental results and density functional theory calculations confirm that the constructed heterostructure and oxygen vacancies optimize the electronic band structure of NiO/NiMoO4–x with more electronic states near the Fermi level, which not only enhances its conductivity, but also promotes exposure of the active sites. Based on this, NiO/NiMoO4–x possesses an impressive OER overpotential of 332 mV and HER overpotential of 34 mV at 10 mA cm–2, simultaneously, a satisfactory stability after continuous operation for 165 h. This work affords valuable insights into the development of durable and inexpensive bifunctional catalysts for electrocatalytic water splitting.
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- article
- Language
- en
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- https://doi.org/10.1016/j.nxnano.2025.100173
- OA Status
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- 50
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- https://openalex.org/W4409906796
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https://openalex.org/W4409906796Canonical identifier for this work in OpenAlex
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https://doi.org/10.1016/j.nxnano.2025.100173Digital Object Identifier
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Manipulating electronic band of NiO/NiMoO4–x nanosheets as robust bifunctional catalyst for water splittingWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-01-01Full publication date if available
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Qiyu Liu, Jintao Zhang, Jingwen He, Peng Zhang, Zujin Yang, Xihong LuList of authors in order
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https://doi.org/10.1016/j.nxnano.2025.100173Publisher landing page
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diamondOpen access status per OpenAlex
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https://doi.org/10.1016/j.nxnano.2025.100173Direct OA link when available
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Bifunctional, Non-blocking I/O, Water splitting, Catalysis, Materials science, Chemical engineering, Nanotechnology, Chemistry, Engineering, Organic chemistry, PhotocatalysisTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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| abstract_inverted_index.structure | 75 |
| abstract_inverted_index.vacancies | 70 |
| abstract_inverted_index.(OER/HER). | 27 |
| abstract_inverted_index.NiO/NiMoO4 | 34 |
| abstract_inverted_index.commercial | 47 |
| abstract_inverted_index.continuous | 127 |
| abstract_inverted_index.electronic | 73, 80 |
| abstract_inverted_index.functional | 60 |
| abstract_inverted_index.impressive | 106 |
| abstract_inverted_index.pollution, | 9 |
| abstract_inverted_index.splitting. | 149 |
| abstract_inverted_index.constructed | 66 |
| abstract_inverted_index.demonstrate | 30 |
| abstract_inverted_index.development | 139 |
| abstract_inverted_index.inexpensive | 143 |
| abstract_inverted_index.bifunctional | 19, 37, 144 |
| abstract_inverted_index.calculations | 62 |
| abstract_inverted_index.experimental | 56 |
| abstract_inverted_index.satisfactory | 124 |
| abstract_inverted_index.vacancy-rich | 33 |
| abstract_inverted_index.conductivity, | 91 |
| abstract_inverted_index.environmental | 8 |
| abstract_inverted_index.overpotential | 108, 114 |
| abstract_inverted_index.NiO/NiMoO4–x | 77, 103 |
| abstract_inverted_index.heterojunction | 35 |
| abstract_inverted_index.NiO/NiMoO4–x) | 45 |
| abstract_inverted_index.environmentally | 15 |
| abstract_inverted_index.heterostructure | 67 |
| abstract_inverted_index.simultaneously, | 122 |
| abstract_inverted_index.electrocatalytic | 40, 147 |
| abstract_inverted_index.hydrothermal-calcination | 53 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 6 |
| citation_normalized_percentile.value | 0.12060165 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |