Manipulating Ferroelectric Topological Polar Structures with Twisted Light Article Swipe
Nimish P. Nazirkar
,
Viet Tran
,
Pascal Bassène
,
Atoumane Ndiaye
,
Julie Barringer
,
Jie Jiang
,
Wonsuk Cha
,
Ross Harder
,
Jian Shi
,
Moussa N’Gom
,
Edwin Fohtung
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202415231
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202415231
The dynamic control of non‐equilibrium states represents a central challenge in condensed matter physics. While intense terahertz fields drive metal‐insulator transitions and ferroelectricity via soft phonon modes, recent theory suggests that twisted light with orbital angular momentum (OAM) offers a distinct route to manipulate ferroelectric order and stabilize topological excitations including skyrmions, vortices, and Hopfions. Control of ferroelectric polarization in quasi‐2D CsBiNb 2 O 7 (CBNO) is demonstrated using non‐resonant twisted ultra‐violet (UV) light (375 nm, 800 THz). Combining in situ X‐ray Bragg coherent diffractive imaging (BCDI), twisted optical Raman spectroscopy, and density functional theory (DFT), three‐dimensional (3D) ionic displacements, strain fields, and polarization changes are resolved in single crystals. Operando measurements reveal light‐induced strain hysteresis under twisted light–a hallmark of nonlinear, history‐dependent ferroelastic switching driven by OAM. Discrete, irreversible domain transitions emerge as the topological charge ℓ is cycled, stabilizing non‐trivial domain textures including vortex‐antivortex pairs, Bloch/anti‐Bloch points, and merons. These persist after OAM removal, indicating a memory effect. Competing mechanisms are discussed, including multiphoton absorption, strain‐mediated polarization switching, and defect‐wall interactions. The findings establish structured light as a tool for deterministic, reversible control of ferroic states, enabling optically reconfigurable non‐volatile devices.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202415231
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202415231
- OA Status
- hybrid
- Cited By
- 2
- References
- 59
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4411089760
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4411089760Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202415231Digital Object Identifier
- Title
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Manipulating Ferroelectric Topological Polar Structures with Twisted LightWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-06-06Full publication date if available
- Authors
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Nimish P. Nazirkar, Viet Tran, Pascal Bassène, Atoumane Ndiaye, Julie Barringer, Jie Jiang, Wonsuk Cha, Ross Harder, Jian Shi, Moussa N’Gom, Edwin FohtungList of authors in order
- Landing page
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https://doi.org/10.1002/adma.202415231Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202415231Direct link to full text PDF
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adma.202415231Direct OA link when available
- Concepts
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Ferroelectricity, Polarization (electrochemistry), Condensed matter physics, Materials science, Topological defect, Raman spectroscopy, Physics, Optics, Optoelectronics, Dielectric, Physical chemistry, ChemistryTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2025: 2Per-year citation counts (last 5 years)
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59Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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