Mapping Phonon Polaritons with Visible Light Article Swipe
Joseph G. Tischler
,
Kiernan E. Arledge
,
Chase T. Ellis
,
Nazli Sarabi
,
Vincent R. Whiteside
,
Chul Han Kim
,
Mijin Kim
,
Daniel Ratchford
,
Michael A. Meeker
,
Binbin Weng
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-4208764/v1
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-4208764/v1
Phonon polaritons (PhPs) are hybrid photon-phonon waves which enable strong light-matter interactions and subdiffractional confinement, potentially empowering applications in sensing, nonlinear optics and nanoscale energy manipulation. In this work, we use confocal Raman microscopy to investigate the coupling between bulk phonon modes and localized surface phonon polariton (SPhP) modes in indium phosphide (InP) nanopillars and 4H-silicon carbide (4H-SiC) gratings. The Raman intensity within the nanostructures is described in terms of the SPhP eigenmodes and used to reconstruct the field intensity, providing a method to map SPhP eigenmodes using visible and near-IR light. Our results indicate that, contrary to expectation, all Raman-active bulk phonon modes of InP and 4H-SiC couple to the localized SPhP modes. Further, we confirm that polarizability selection rules form the predominant coupling mechanism between phonons and SPhP modes, with electron-phonon coupling playing a role for certain phonon modes (A1(LO) and E1(TO) in 4H-SiC). These observations provide a method for extending Raman studies of PhP modes to achieve full 3D reconstruction of the PhP eigenmodes and visualize light-matter interactions within nanostructures, thus advancing Raman scattering as a technique for understanding PhP modes.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-4208764/v1
- https://www.researchsquare.com/article/rs-4208764/latest.pdf
- OA Status
- gold
- References
- 38
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4398255429
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Raw OpenAlex JSON
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https://openalex.org/W4398255429Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.21203/rs.3.rs-4208764/v1Digital Object Identifier
- Title
-
Mapping Phonon Polaritons with Visible LightWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-05-23Full publication date if available
- Authors
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Joseph G. Tischler, Kiernan E. Arledge, Chase T. Ellis, Nazli Sarabi, Vincent R. Whiteside, Chul Han Kim, Mijin Kim, Daniel Ratchford, Michael A. Meeker, Binbin WengList of authors in order
- Landing page
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https://doi.org/10.21203/rs.3.rs-4208764/v1Publisher landing page
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https://www.researchsquare.com/article/rs-4208764/latest.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.researchsquare.com/article/rs-4208764/latest.pdfDirect OA link when available
- Concepts
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Phonon, Raman spectroscopy, Polariton, Raman scattering, Surface phonon, Nanopillar, Coupling (piping), Optoelectronics, Condensed matter physics, Materials science, Physics, Optics, Nanostructure, Nanotechnology, MetallurgyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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38Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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