Mechanism of Electron Spin Decoherence in a Partially Deuterated Glassy Matrix Article Swipe
Samuel M. Jahn
,
Elizabeth R. Canarie
,
Stefan Stoll
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpclett.2c00939
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpclett.2c00939
Long electron spin coherence lifetimes are essential for applications in quantum information science and electron paramagnetic resonance, for instance, for nanoscale distance measurements in biomolecular systems using double electron-electron resonance. We experimentally investigate the decoherence dynamics under the Hahn echo sequence of the organic radical d18-TEMPO in a variably deuterated frozen water:glycerol matrix. The coherence time (phase memory time) TM scales with proton concentration as [1H]-0.65. For selectively deuterated matrices, decoherence is accelerated in the presence of proton clustering, that is, substantial short-range density in the proton-proton radial distribution functions (2 and OH2 groups are major decoherence drivers. This provides a predictive tool for designing molecular systems with long electron spin coherence times.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.jpclett.2c00939
- OA Status
- green
- Cited By
- 27
- References
- 42
- Related Works
- 10
- OpenAlex ID
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https://openalex.org/W4281642180Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.jpclett.2c00939Digital Object Identifier
- Title
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Mechanism of Electron Spin Decoherence in a Partially Deuterated Glassy MatrixWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-06-10Full publication date if available
- Authors
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Samuel M. Jahn, Elizabeth R. Canarie, Stefan StollList of authors in order
- Landing page
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https://doi.org/10.1021/acs.jpclett.2c00939Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
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https://www.ncbi.nlm.nih.gov/pmc/articles/9503049Direct OA link when available
- Concepts
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Quantum decoherence, Proton, Electron, Coherence (philosophical gambling strategy), Deuterium, Spin (aerodynamics), Geminal, Physics, Electron paramagnetic resonance, Density matrix, Quantum, Atomic physics, Chemistry, Chemical physics, Nuclear magnetic resonance, Quantum mechanics, Thermodynamics, StereochemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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27Total citation count in OpenAlex
- Citations by year (recent)
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2025: 10, 2024: 9, 2023: 8Per-year citation counts (last 5 years)
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42Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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