Mechanisms of degradation of polycyclic aromatic hydrocarbons by biochar and biochar-mineral composites in the dry system Article Swipe
Pengfei Cheng
,
Haoli Qin
,
Juan Cheng
,
Junliang Chen
,
Miao Yu
,
Zhiliang Li
,
Lu Yao
,
Guanlin Li
,
Daolin Du
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.apcato.2025.207047
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.apcato.2025.207047
Polycyclic aromatic hydrocarbons (PAHs) are widely distributed in arid/semi-arid soils, and their hydrophobicity and bioaccumulation pose significant threats to ecosystems and human health. Conventional remediation techniques such as advanced oxidation, are limited by high costs and secondary contamination risks, driving the need for efficient and eco-friendly in-situ methods. In this study, the activity of biochar derived from invasive plant Wedelia trilobata (pyrolyzed at 400, 600, and 800 °C; BC400/600/800) were assessed by BET, XPS, CV, and EPR. The efficacy of biochar-mineral (goethite, hematite, magnetite, birnessite, cryptomelane, montmorillonite, and kaolinite) composites for PAHs degradation performance and the mechanisms were studied. BC800 was optimal for benzo(a)pyrene (BaP) degradation (rate constant: 0.0360 min−1), attributable to its high specific surface area (301.44 m2/g), abundant oxygen-containing functional groups (CO, CO), and electron transfer capacity. The degradation rates were positively correlated with the highest occupied molecular orbital (HOMO) levels of the PAHs (R2 = 0.6850), confirming dominant electron transfer. Among seven mineral composites, the Bir-biochar combination enhanced BaP degradation by 2.3-fold through the “electron shuttle” function of the Mn(IV)/Mn(III) redox couples. In a dry system, as the moisture increased, the degradation efficiency also increased. This study elucidates the adsorption-electron transfer mechanism of biochar-mineral composites for PAHs degradation in arid environments, providing a theoretical foundation and technical support for utilizing invasive plants utilization and remediating dryland soils polluted with organic species.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.apcato.2025.207047
- OA Status
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- Cited By
- 2
- References
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- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4409815993Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.apcato.2025.207047Digital Object Identifier
- Title
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Mechanisms of degradation of polycyclic aromatic hydrocarbons by biochar and biochar-mineral composites in the dry systemWork title
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
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2025-04-25Full publication date if available
- Authors
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Pengfei Cheng, Haoli Qin, Juan Cheng, Junliang Chen, Miao Yu, Zhiliang Li, Lu Yao, Guanlin Li, Daolin DuList of authors in order
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https://doi.org/10.1016/j.apcato.2025.207047Publisher landing page
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diamondOpen access status per OpenAlex
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https://doi.org/10.1016/j.apcato.2025.207047Direct OA link when available
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Biochar, Degradation (telecommunications), Mineral, Environmental science, Environmental chemistry, Chemistry, Materials science, Pyrolysis, Metallurgy, Organic chemistry, Computer science, TelecommunicationsTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2025: 2Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.CO), | 124 |
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