Microstructured Macromaterials Based on IPN Microgels Article Swipe
I. R. Nasimova
,
Vladimir Yu. Rudyak
,
Anton Pavlovich Doroganov
,
Elena P. Kharitonova
,
Elena Yu. Kozhunova
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.3390/polym13071078
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.3390/polym13071078
This study investigates the formation of microstructured macromaterials from thermo- and pH-sensitive microgels based on interpenetrating networks of poly-N-isopropylacrylamide (PNIPAM) and polyacrylic acid (PAA). Macromaterials are produced as a result of the deposition of microgel particles and subsequent crosslinking of polyacrylic acid subnetworks to each other due to the formation of the anhydride bonds during annealing. Since both PNIPAM and PAA are environment-sensitive polymers, one can expect that their conformational state during material development will affect its resulting properties. Thus, the influence of conditions of preparation for annealing (pH of the solution, the temperature of preliminary drying) on the swelling behavior, pH- and thermosensitivity, and macromaterial inner structure was investigated. In parallel, the study of the effect of the relative conformations of the IPN microgel subnetworks on the formation of macromaterials was carried out by the computer simulations method. It was shown that the properties of the prepared macromaterials strongly depend both on the temperature and pH of the PNIPAM-PAA IPN microgel dispersions. This opens up new opportunities to obtain materials with pre-chosen characteristics and environmental sensitivity.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/polym13071078
- https://www.mdpi.com/2073-4360/13/7/1078/pdf?version=1617937990
- OA Status
- gold
- Cited By
- 12
- References
- 43
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3147749481
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https://openalex.org/W3147749481Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/polym13071078Digital Object Identifier
- Title
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Microstructured Macromaterials Based on IPN MicrogelsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-03-29Full publication date if available
- Authors
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I. R. Nasimova, Vladimir Yu. Rudyak, Anton Pavlovich Doroganov, Elena P. Kharitonova, Elena Yu. KozhunovaList of authors in order
- Landing page
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https://doi.org/10.3390/polym13071078Publisher landing page
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https://www.mdpi.com/2073-4360/13/7/1078/pdf?version=1617937990Direct link to full text PDF
- Open access
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/2073-4360/13/7/1078/pdf?version=1617937990Direct OA link when available
- Concepts
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Polyacrylic acid, Swelling, Materials science, Polymer, Poly(N-isopropylacrylamide), Chemical engineering, Annealing (glass), Polymer chemistry, Acrylic acid, Interpenetrating polymer network, Network formation, Copolymer, Composite material, World Wide Web, Engineering, Computer scienceTop concepts (fields/topics) attached by OpenAlex
- Cited by
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12Total citation count in OpenAlex
- Citations by year (recent)
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2025: 4, 2024: 1, 2023: 2, 2022: 2, 2021: 3Per-year citation counts (last 5 years)
- References (count)
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43Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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