MIL-100(Fe) /ZnO nanocomposite sensors: An enhanced ammonia selectivity and low operating temperature Article Swipe
Seyed Parsa Amouzesh
,
Abbas Ali Khodadadi
,
Yadollah Mortazavi
,
Seryio Saris
,
Mehrdad Asgari
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1016/j.snb.2023.134791
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1016/j.snb.2023.134791
This study aims to enhance the response and selectivity of zinc oxide (ZnO) gas sensors by its incorporating in MIL-100(Fe) as a support material. ZnO nanocomposites were synthesized by impregnating MIL-100 with varying weight percentages of zinc oxide (10% to 20%). The fabricated sensors underwent characterization through XRD, FTIR, DRS (UV-Vis), SEM/EDS, and NH3-TPD techniques to assess their material composition and sensor performance. DRS (UV-Vis) techniques revealed a significant decrease in the band gap, from Tauc analysis, accompanied by a 20% decrease in the Schottky barrier of the nanocomposite, compare to ZnO. Furthermore, the optimal operating temperature for the MIL-100/ZnO nanocomposites was identified as 240°C, contrasting with pure ZnO sensors that exhibited an increasing response with temperature. Notably, the MIL-100/ZnO nanocomposites exhibited substantially improved selectivity for ammonia, displaying 3 to 6 times higher selectivity compared to pure ZnO sensors. Additionally, the response to ammonia increased threefold in the MIL-100/ZnO nanocomposites. This enhancement in selectivity and response can be attributed to the synergistic interaction between ammonia molecules and the Lewis acid sites present in the MIL-100 framework, facilitated by coordination bonds. The findings underscore the immense potential of MIL-100/ZnO nanocomposites as a promising solution for augmenting the selectivity of ZnO gas sensors. This work contributes valuable insights towards the advancement of gas sensing technology and paves the way for the development of highly selective gas sensors with extensive applications across various fields.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.snb.2023.134791
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- Cited By
- 30
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https://openalex.org/W4387662537Canonical identifier for this work in OpenAlex
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https://doi.org/10.1016/j.snb.2023.134791Digital Object Identifier
- Title
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MIL-100(Fe) /ZnO nanocomposite sensors: An enhanced ammonia selectivity and low operating temperatureWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-10-16Full publication date if available
- Authors
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Seyed Parsa Amouzesh, Abbas Ali Khodadadi, Yadollah Mortazavi, Seryio Saris, Mehrdad AsgariList of authors in order
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https://doi.org/10.1016/j.snb.2023.134791Publisher landing page
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hybridOpen access status per OpenAlex
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https://doi.org/10.1016/j.snb.2023.134791Direct OA link when available
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Nanocomposite, Selectivity, Materials science, Zinc, Ammonia, Graphene, Chemical engineering, Fourier transform infrared spectroscopy, Oxide, Nanotechnology, Chemistry, Catalysis, Organic chemistry, Metallurgy, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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30Total citation count in OpenAlex
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2025: 14, 2024: 16Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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