Modular Design of Functional Glucose Monomer and Block Co‐Polymer toward Stable Zn Anodes Article Swipe
Yaping Yan
,
Ruhuai Mei
,
Jiachen Ma
,
Yang Huang
,
Ying Zhu
,
Zhen Lang
,
Cheng Li
,
Hongmei Tang
,
Wenlan Zhang
,
Jing Lu
,
Oliver G. Schmidt
,
Kai Zhang
,
Minshen Zhu
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/smll.202400292
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/smll.202400292
Aqueous Zn batteries employing mildly acidic electrolytes have emerged as promising contenders for safe and cost‐effective energy storage solutions. Nevertheless, the intrinsic reversibility of the Zn anode becomes a focal concern due to the involvement of acidic electrolyte, which triggers Zn corrosion and facilitates the deposition of insulating byproducts. Moreover, the unregulated growth of Zn over cycling amplifies the risk of internal short‐circuiting, primarily induced by the formation of Zn dendrites. In this study, a class of glucose‐derived monomers and a block copolymer are synthesized through a building‐block assembly strategy, ultimately leading to uncover the optimal polymer structure that suppresses the Zn corrosion while allowing efficient ion conduction with a substantial contribution from cation transport. Leveraging these advancements, remarkable enhancements are achieved in the realm of Zn reversibility, exemplified by a spectrum of performance metrics, including robust cycling stability without voltage overshoot and short‐circuiting during 3000 h of cycling, stable operation at a high depth of charge/discharge of 75% and a high current density, >95% Coulombic efficiency over 2000 cycles, successful translation of the anode improvement to full cell performance. These polymer designs offer a transformative path based on the modular synthesis of polymeric coatings toward highly reversible Zn anode.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/smll.202400292
- OA Status
- hybrid
- Cited By
- 9
- References
- 60
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4395455882
All OpenAlex metadata
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https://openalex.org/W4395455882Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/smll.202400292Digital Object Identifier
- Title
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Modular Design of Functional Glucose Monomer and Block Co‐Polymer toward Stable Zn AnodesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-04-25Full publication date if available
- Authors
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Yaping Yan, Ruhuai Mei, Jiachen Ma, Yang Huang, Ying Zhu, Zhen Lang, Cheng Li, Hongmei Tang, Wenlan Zhang, Jing Lu, Oliver G. Schmidt, Kai Zhang, Minshen ZhuList of authors in order
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https://doi.org/10.1002/smll.202400292Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1002/smll.202400292Direct OA link when available
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Modular design, Monomer, Anode, Polymer, Materials science, Chemical engineering, Block (permutation group theory), Electrode, Nanotechnology, Chemistry, Computer science, Composite material, Mathematics, Engineering, Physical chemistry, Operating system, GeometryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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9Total citation count in OpenAlex
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2025: 7, 2024: 2Per-year citation counts (last 5 years)
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60Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.electrolytes | 7 |
| abstract_inverted_index.enhancements | 120 |
| abstract_inverted_index.performance. | 180 |
| abstract_inverted_index.Nevertheless, | 20 |
| abstract_inverted_index.advancements, | 118 |
| abstract_inverted_index.reversibility | 23 |
| abstract_inverted_index.reversibility, | 128 |
| abstract_inverted_index.transformative | 186 |
| abstract_inverted_index.building‐block | 88 |
| abstract_inverted_index.charge/discharge | 157 |
| abstract_inverted_index.cost‐effective | 16 |
| abstract_inverted_index.glucose‐derived | 78 |
| abstract_inverted_index.short‐circuiting | 144 |
| abstract_inverted_index.short‐circuiting, | 63 |
| cited_by_percentile_year.max | 99 |
| cited_by_percentile_year.min | 94 |
| countries_distinct_count | 3 |
| institutions_distinct_count | 13 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
| sustainable_development_goals[0].score | 0.8799999952316284 |
| sustainable_development_goals[0].display_name | Affordable and clean energy |
| citation_normalized_percentile.value | 0.89580983 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |