Modulating selective interaction of NiOOH with Mg ions for high-performance aqueous batteries Article Swipe
Bing He
,
Ying Ling
,
Zhixun Wang
,
Wenbin Gong
,
Zhe Wang
,
Yanting Liu
,
Tianzhu Zhou
,
Ting Xiong
,
Shuai Wang
,
Yonggang Wang
,
Qingwen Li
,
Qichong Zhang
,
Lei Wei
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1016/j.esci.2024.100293
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1016/j.esci.2024.100293
Aqueous Mg-ion batteries (AMIBs) featuring advantages of good safety, low cost, and high specific energy have been recognized as a promising energy-storage technology. However, the performance of AMIBs is consistently limited by sluggish diffusion kinetics and structural degradation of cathode materials arising from the strong electrostatic interactions between high-charge-density Mg2+ and host materials. Here, layered-structured NiOOH, as traditional cathodes for alkaline batteries, is initially demonstrated to realize proton-assisted Mg-(de)intercalation chemistry with a high discharge platform (0.57 V) in neutral aqueous electrolytes. Benefiting from the unique core/shell structure, the resulting NiOOH/CNT cathodes achieve a high capacity of 122.5 mAh g−1 and long cycle stability. Further theoretical calculations reveal that the binding energy of hydrated Mg2+ is higher than that of Mg2+ with NiOOH, resulting in that Mg2+ is easily intercalated/de-intercalated into/from NiOOH. Benefiting from the freestanding design, the assembled fiber-shaped “rocking-chair” NaTi2(PO4)3//NiOOH AMIB shows a high energy density and satisfactory mechanical flexibility, which could be woven into a commercial fabric and power for fiber-shaped photoelectric sensors.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.esci.2024.100293
- OA Status
- gold
- Cited By
- 38
- References
- 67
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4399914585
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4399914585Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.esci.2024.100293Digital Object Identifier
- Title
-
Modulating selective interaction of NiOOH with Mg ions for high-performance aqueous batteriesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
-
2024-06-22Full publication date if available
- Authors
-
Bing He, Ying Ling, Zhixun Wang, Wenbin Gong, Zhe Wang, Yanting Liu, Tianzhu Zhou, Ting Xiong, Shuai Wang, Yonggang Wang, Qingwen Li, Qichong Zhang, Lei WeiList of authors in order
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https://doi.org/10.1016/j.esci.2024.100293Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1016/j.esci.2024.100293Direct OA link when available
- Concepts
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Cathode, Intercalation (chemistry), Aqueous solution, Electrolyte, Materials science, Chemical engineering, Ion, Power density, Energy storage, Battery (electricity), Nanotechnology, Chemistry, Inorganic chemistry, Electrode, Physical chemistry, Power (physics), Organic chemistry, Thermodynamics, Physics, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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38Total citation count in OpenAlex
- Citations by year (recent)
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2025: 35, 2024: 3Per-year citation counts (last 5 years)
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67Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| citation_normalized_percentile.value | 0.98875248 |
| citation_normalized_percentile.is_in_top_1_percent | True |
| citation_normalized_percentile.is_in_top_10_percent | True |