Molecular Engineering of Coacervate Network Binders for Stable Silicon‐Based Anodes in Lithium‐Ion Batteries Article Swipe
Dong‐Yeob Han
,
Im Kyung Han
,
Junsu Son
,
Jin Yong Kwon
,
Youn Soo Kim
,
Tae Kyung Lee
,
Soo‐Jin Park
,
Jaegeon Ryu
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202509445
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202509445
The growing demand for high‐energy‐density lithium‐ion batteries (LIBs) has spurred interest in silicon (Si)‐based anodes, but their practical use is hindered by volumetric expansion during cycling, leading to electrode degradation and uncontrolled solid electrolyte interphase (SEI) growth. Here, a molecularly engineered approach is presented to regulate Coulomb interactions in coacervate charged polymer binders for stabilizing Si anodes. By systematically tuning effective charge density through different functional groups, electrostatic interactions within the binder network are modulated to optimize adhesion, mechanical integrity, and electrochemical performance. Four charged polymers with varying functional groups: amine (A), guanidine (G), sulfonate (S), and carboxylate (C) are synthesized and studied. The G‐C binder, exhibiting the strongest Coulomb interaction, demonstrated superior adhesion, mechanical stability, and cycling performance. This binder enabled the fabrication of ultra‐high areal capacity Si‐based electrodes (12.2 mAh cm −2 ), outperforming previously reported binder systems. Moreover, full‐cell evaluations of Si‐based anodes with G‐C binders and Ni‐rich layered cathodes demonstrated stable cycling at high areal capacities (4.7 mAh cm −2 ), underscoring the practical viability of this approach. These findings establish Coulomb interactions as a key design parameter for next‐generation polymer binders, offering a promising strategy to address the long‐standing challenges of Si‐based anodes in LIBs.
Related Topics
Concepts
Materials science
Anode
Silicon
Coacervate
Lithium (medication)
Ion
Nanotechnology
Nanoarchitectures for lithium-ion batteries
Chemical engineering
Metallurgy
Electrode
Organic chemistry
Physical chemistry
Endocrinology
Chemistry
Engineering
Medicine
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adfm.202509445
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202509445
- OA Status
- hybrid
- Cited By
- 2
- References
- 43
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4412372695
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4412372695Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adfm.202509445Digital Object Identifier
- Title
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Molecular Engineering of Coacervate Network Binders for Stable Silicon‐Based Anodes in Lithium‐Ion BatteriesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-06-29Full publication date if available
- Authors
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Dong‐Yeob Han, Im Kyung Han, Junsu Son, Jin Yong Kwon, Youn Soo Kim, Tae Kyung Lee, Soo‐Jin Park, Jaegeon RyuList of authors in order
- Landing page
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https://doi.org/10.1002/adfm.202509445Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202509445Direct link to full text PDF
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202509445Direct OA link when available
- Concepts
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Materials science, Anode, Silicon, Coacervate, Lithium (medication), Ion, Nanotechnology, Nanoarchitectures for lithium-ion batteries, Chemical engineering, Metallurgy, Electrode, Organic chemistry, Physical chemistry, Endocrinology, Chemistry, Engineering, MedicineTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2Per-year citation counts (last 5 years)
- References (count)
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43Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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