Monolithic dynamic covalent polymer aerogels via ambient pressure drying with super-flexibility, weldability, closed-loop recyclability, and multifunctionality Article Swipe
Xinhai Zhang
,
Jun Zhao
,
Kai Liu
,
Guangfeng Li
,
Dong Zhao
,
Zhaoming Zhao
,
Junjun Wan
,
Xue Yang
,
Ruixue Bai
,
Yongming Wang
,
Wei Zhang
,
Xuzhou Yan
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2021-gxp40
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.26434/chemrxiv-2021-gxp40
Owing to their low density, high porosity and unique micro-nanostructures, aerogels are attractive for applications in various aspects, but at the same time, suffer from shrinkage and/or cracking during preparation, mechanical brittleness, low production efficiency, and non-degradation. Herein, we introduce the concept of dynamic covalent polymer chemistry to produce a new class of aerogelsreferred to as DCPAs. The resulting light DCPAs display large-scale preparation prospect and feature high porosity (90.7-91.3%), large degrees of compression (80% strain) and bending (diametral deflection of 30 mm) without any cracks, as well as considerable tensile property (elongation at break of 32.7%). In addition, our DCPAs showcase emergent characteristics of weldability, repairability, and closed-loop recyclability that are highly desirable for affording versatile materials platforms but hardly achieved by traditional aerogels. Benefiting from the robust porous structures, we demonstrate the potential of the DCPAs for applications in thermal insulation and emulsion separation.
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- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.26434/chemrxiv-2021-gxp40
- https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/60cbf142926ad0487a01becf/original/monolithic-dynamic-covalent-polymer-aerogels-via-ambient-pressure-drying-with-super-flexibility-weldability-closed-loop-recyclability-and-multifunctionality.pdf
- OA Status
- gold
- References
- 47
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4230480209
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- OpenAlex ID
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https://openalex.org/W4230480209Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.26434/chemrxiv-2021-gxp40Digital Object Identifier
- Title
-
Monolithic dynamic covalent polymer aerogels via ambient pressure drying with super-flexibility, weldability, closed-loop recyclability, and multifunctionalityWork title
- Type
-
preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
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2021Year of publication
- Publication date
-
2021-06-21Full publication date if available
- Authors
-
Xinhai Zhang, Jun Zhao, Kai Liu, Guangfeng Li, Dong Zhao, Zhaoming Zhao, Junjun Wan, Xue Yang, Ruixue Bai, Yongming Wang, Wei Zhang, Xuzhou YanList of authors in order
- Landing page
-
https://doi.org/10.26434/chemrxiv-2021-gxp40Publisher landing page
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https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/60cbf142926ad0487a01becf/original/monolithic-dynamic-covalent-polymer-aerogels-via-ambient-pressure-drying-with-super-flexibility-weldability-closed-loop-recyclability-and-multifunctionality.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/60cbf142926ad0487a01becf/original/monolithic-dynamic-covalent-polymer-aerogels-via-ambient-pressure-drying-with-super-flexibility-weldability-closed-loop-recyclability-and-multifunctionality.pdfDirect OA link when available
- Concepts
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Materials science, Weldability, Porosity, Composite material, Ultimate tensile strength, Polymer, Brittleness, Toughness, Cracking, WeldingTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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