Monoterpene chemical speciation in the Amazon tropical rainforest: variation with season, height, and time of day at the Amazon Tall Tower Observatory (ATTO) Article Swipe
Ana María Yáñez‐Serrano
,
A. C. Nölscher
,
Efstratios Bourtsoukidis
,
Eliane Gomes Alves
,
L. Ganzeveld
,
Boris Bonn
,
Stefan Wolff
,
Marta Sá
,
Márcia Akemi Yamasoe
,
Jonathan Williams
,
Meinrat O. Andreae
,
J. Kesselmeier
·
YOU?
·
· 2017
· Open Access
·
· DOI: https://doi.org/10.5194/acp-2017-817
YOU?
·
· 2017
· Open Access
·
· DOI: https://doi.org/10.5194/acp-2017-817
Speciated monoterpene measurements in the Amazon rainforest air are scarce, but important in order to understand their contribution to the overall reactivity of volatile organic compound (VOCs) emissions towards the main atmospheric oxidants, such as hydroxyl radical (OH), ozone (O3) and nitrate radical (NO3). In this study, we present the chemical speciation of gas phase monoterpenes measured in the tropical rainforest at the Amazon Tall Tower Observatory (ATTO, Amazonas, Brazil). Samples of VOCs were collected by two automatic sampling systems positioned on a tower at 12 and 24 m height and analysed using Gas Chromatography Flame Ionization Detection (GC-FID). The samples were collected in October 2015, representing the dry season, and compared with previous wet and dry season studies at the site. In addition, vertical profile measurements (at 12 and 24 m) of total monoterpene mixing ratios were made using Proton-Transfer Reaction Mass Spectrometry (PTR-MS). The results showed a distinctly different chemical speciation between day and night. For instance, α-pinene was more abundant during the day, whereas limonene was more abundant at night. Reactivity calculations showed that the most abundant compounds may not be the most atmospheric chemically relevant compounds. Furthermore, inter- and intra-annual results demonstrate similar chemodiversity during the dry seasons analysed. Simulations with a canopy exchange modelling system compare relatively well with the observed temporal variability in speciated monoterpene mixing ratios, but also indicate the necessity of more experiments to enhance our understanding of in-canopy sinks of these monoterpenes.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.5194/acp-2017-817
- OA Status
- gold
- Cited By
- 1
- References
- 56
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4250054247
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4250054247Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.5194/acp-2017-817Digital Object Identifier
- Title
-
Monoterpene chemical speciation in the Amazon tropical rainforest: variation with season, height, and time of day at the Amazon Tall Tower Observatory (ATTO)Work title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2017Year of publication
- Publication date
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2017-09-19Full publication date if available
- Authors
-
Ana María Yáñez‐Serrano, A. C. Nölscher, Efstratios Bourtsoukidis, Eliane Gomes Alves, L. Ganzeveld, Boris Bonn, Stefan Wolff, Marta Sá, Márcia Akemi Yamasoe, Jonathan Williams, Meinrat O. Andreae, J. KesselmeierList of authors in order
- Landing page
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https://doi.org/10.5194/acp-2017-817Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.5194/acp-2017-817Direct OA link when available
- Concepts
-
Monoterpene, Amazon rainforest, Dry season, Aerosol, Environmental chemistry, Chemistry, Atmospheric sciences, Atmospheric chemistry, Environmental science, Ozone, Rainforest, Botany, Ecology, Biology, Organic chemistry, GeologyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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1Total citation count in OpenAlex
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2023: 1Per-year citation counts (last 5 years)
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56Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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