Motility-induced Phase Separation is Reentrant Article Swipe
Zhonghuai Hou
,
Huijun Jiang
,
Meng-Kai Feng
,
Jie Su
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-1621424/v1
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-1621424/v1
Active Brownian particles (ABPs) with pure repulsion is an ideal model to understand the effect of nonequilibrium on collective behaviors. It has long been established that activity can create effective attractions leading to motility-induced phase separation (MIPS), whose role is similar to that of (inverse) temperature in the simplest equilibrium system with attractive inter-particle interactions. Here, we report both theoretically and numerically that activity can lead to a counterintuitive MIPS reentrance, which is completely different from the phase behavior of equilibrium systems. Our theoretical analysis based on a kinetic theory of MIPS shows that a new type of activity-induced nonequilibrium vaporization is able to hinder the formation of dense phase when activity is large enough. Such nonequilibrium vaporization along with the activity-induced effective attraction thus lead to the MIPS reentrance. Numerical simulations verify such nonequilibrium effect induced solely by activity on phase behaviors of ABPs, and further demonstrate the dependence of MIPS on activity and the strength of inter-particle interaction predicted by our theoretical analysis. Our findings highlight the unique role played by the nonequilibrium nature of activity on phase behaviors of active systems, which may inspire deep insights into the essential difference between equilibrium and nonequilibrium systems.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-1621424/v1
- https://www.researchsquare.com/article/rs-1621424/latest.pdf
- OA Status
- green
- References
- 37
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4280607290
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4280607290Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.21203/rs.3.rs-1621424/v1Digital Object Identifier
- Title
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Motility-induced Phase Separation is ReentrantWork title
- Type
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preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-05-12Full publication date if available
- Authors
-
Zhonghuai Hou, Huijun Jiang, Meng-Kai Feng, Jie SuList of authors in order
- Landing page
-
https://doi.org/10.21203/rs.3.rs-1621424/v1Publisher landing page
- PDF URL
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https://www.researchsquare.com/article/rs-1621424/latest.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://www.researchsquare.com/article/rs-1621424/latest.pdfDirect OA link when available
- Concepts
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Non-equilibrium thermodynamics, Brownian dynamics, Phase (matter), Statistical physics, Metastability, Particle (ecology), Reentrancy, Brownian motion, Physics, Materials science, Chemical physics, Thermodynamics, Condensed matter physics, Quantum mechanics, Geology, OceanographyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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37Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| primary_location.pdf_url | https://www.researchsquare.com/article/rs-1621424/latest.pdf |
| primary_location.version | acceptedVersion |
| primary_location.raw_type | posted-content |
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| publication_date | 2022-05-12 |
| publication_year | 2022 |
| referenced_works | https://openalex.org/W3037683188, https://openalex.org/W2912918439, https://openalex.org/W2979408268, https://openalex.org/W3102746675, https://openalex.org/W3148287403, https://openalex.org/W1999377530, https://openalex.org/W2006628332, https://openalex.org/W2292328547, https://openalex.org/W4299516620, https://openalex.org/W1836107020, https://openalex.org/W3100638106, https://openalex.org/W2001409136, https://openalex.org/W1660598416, https://openalex.org/W2076797206, https://openalex.org/W2913663338, https://openalex.org/W3120896048, https://openalex.org/W3037030126, https://openalex.org/W2592275661, https://openalex.org/W2489784754, https://openalex.org/W2091968362, https://openalex.org/W2005751229, https://openalex.org/W2528272087, https://openalex.org/W2021699244, https://openalex.org/W2593003188, https://openalex.org/W2001008633, https://openalex.org/W2894751282, https://openalex.org/W2468824508, https://openalex.org/W3121989870, https://openalex.org/W3035396425, https://openalex.org/W3006685803, https://openalex.org/W2304845716, https://openalex.org/W2074291204, https://openalex.org/W2131119017, https://openalex.org/W2153920886, https://openalex.org/W2807759594, https://openalex.org/W3104310224, https://openalex.org/W1971373010 |
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