Multidimensional thermally-induced transformation of nest-structured\n complex Au-Fe nanoalloys towards equilibrium Article Swipe
Jacob Johny
,
Oleg Prymak
,
Marius Kamp
,
F. Calvo
,
Se‐Ho Kim
,
Anna Tymoczko
,
Ayman A. El‐Zoka
,
Christoph Rehbock
,
Ulrich Schürmann
,
Baptiste Gault
,
Lorenz Kienle
,
Stephan Barcikowski
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2104.13491
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2104.13491
Bimetallic nanoparticles are often superior candidates for a wide range of\ntechnological and biomedical applications, thanks to their enhanced catalytic,\noptical, and magnetic properties, which are often better than their\nmonometallic counterparts. Most of their properties strongly depend on their\nchemical composition, crystallographic structure, and phase distribution.\nHowever, little is known of how their crystal structure, on the nanoscale,\ntransforms over time at elevated temperatures, even though this knowledge is\nhighly relevant in case nanoparticles are used in, e.g., high-temperature\ncatalysis. Au-Fe is a promising bimetallic system where the low-cost and\nmagnetic Fe is combined with catalytically active and plasmonic Au. Here, we\nreport on the in situ temporal evolution of the crystalline ordering in Au-Fe\nnanoparticles, obtained from a modern laser ablation in liquids synthesis. Our\nin-depth analysis, complemented by dedicated atomistic simulations, includes a\ndetailed structural characterization by X-ray diffraction and transmission\nelectron microscopy as well as atom probe tomography to reveal elemental\ndistributions down to a single atom resolution. We show that the Au-Fe\nnanoparticles initially exhibit highly complex internal nested nanostructures\nwith a wide range of compositions, phase distributions, and size-depended\nmicrostrains. The elevated temperature induces a diffusion-controlled\nrecrystallization and phase merging, resulting in the formation of a single\nface-centered-cubic ultrastructure in contact with a body-centered cubic phase,\nwhich demonstrates the metastability of these structures. Uncovering these\nunique nanostructures with nested features could be highly attractive from a\nfundamental viewpoint as they could give further insights into the nanoparticle\nformation mechanism under non-equilibrium conditions.\n
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2104.13491
- https://arxiv.org/pdf/2104.13491
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4287199305
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4287199305Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2104.13491Digital Object Identifier
- Title
-
Multidimensional thermally-induced transformation of nest-structured\n complex Au-Fe nanoalloys towards equilibriumWork title
- Type
-
preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-04-27Full publication date if available
- Authors
-
Jacob Johny, Oleg Prymak, Marius Kamp, F. Calvo, Se‐Ho Kim, Anna Tymoczko, Ayman A. El‐Zoka, Christoph Rehbock, Ulrich Schürmann, Baptiste Gault, Lorenz Kienle, Stephan BarcikowskiList of authors in order
- Landing page
-
https://arxiv.org/abs/2104.13491Publisher landing page
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https://arxiv.org/pdf/2104.13491Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://arxiv.org/pdf/2104.13491Direct OA link when available
- Concepts
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Materials science, Nanoparticle, Bimetallic strip, Nanostructure, Metastability, Atom probe, Phase (matter), Transmission electron microscopy, Nanotechnology, Nanoscopic scale, Atom (system on chip), Chemical physics, Crystallography, Chemistry, Metal, Metallurgy, Embedded system, Computer science, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.case | 66 |
| abstract_inverted_index.down | 141 |
| abstract_inverted_index.even | 59 |
| abstract_inverted_index.from | 107, 208 |
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| abstract_inverted_index.time | 55 |
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| abstract_inverted_index.well | 133 |
| abstract_inverted_index.wide | 8, 160 |
| abstract_inverted_index.with | 86, 187, 201 |
| abstract_inverted_index.Au-Fe | 73 |
| abstract_inverted_index.Here, | 92 |
| abstract_inverted_index.X-ray | 127 |
| abstract_inverted_index.could | 204, 213 |
| abstract_inverted_index.cubic | 190 |
| abstract_inverted_index.e.g., | 71 |
| abstract_inverted_index.known | 45 |
| abstract_inverted_index.laser | 110 |
| abstract_inverted_index.often | 3, 24 |
| abstract_inverted_index.phase | 41, 164, 175 |
| abstract_inverted_index.probe | 136 |
| abstract_inverted_index.range | 9, 161 |
| abstract_inverted_index.their | 16, 31, 48 |
| abstract_inverted_index.these | 196 |
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| abstract_inverted_index.which | 22 |
| abstract_inverted_index.active | 88 |
| abstract_inverted_index.better | 25 |
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| abstract_inverted_index.highly | 154, 206 |
| abstract_inverted_index.little | 43 |
| abstract_inverted_index.modern | 109 |
| abstract_inverted_index.nested | 157, 202 |
| abstract_inverted_index.reveal | 139 |
| abstract_inverted_index.single | 144 |
| abstract_inverted_index.system | 78 |
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| abstract_inverted_index.though | 60 |
| abstract_inverted_index.complex | 155 |
| abstract_inverted_index.contact | 186 |
| abstract_inverted_index.crystal | 49 |
| abstract_inverted_index.exhibit | 153 |
| abstract_inverted_index.further | 215 |
| abstract_inverted_index.induces | 171 |
| abstract_inverted_index.liquids | 113 |
| abstract_inverted_index.ablation | 111 |
| abstract_inverted_index.combined | 85 |
| abstract_inverted_index.elevated | 57, 169 |
| abstract_inverted_index.enhanced | 17 |
| abstract_inverted_index.features | 203 |
| abstract_inverted_index.includes | 122 |
| abstract_inverted_index.insights | 216 |
| abstract_inverted_index.internal | 156 |
| abstract_inverted_index.low-cost | 81 |
| abstract_inverted_index.magnetic | 20 |
| abstract_inverted_index.merging, | 176 |
| abstract_inverted_index.obtained | 106 |
| abstract_inverted_index.ordering | 103 |
| abstract_inverted_index.relevant | 64 |
| abstract_inverted_index.strongly | 33 |
| abstract_inverted_index.superior | 4 |
| abstract_inverted_index.temporal | 98 |
| abstract_inverted_index.analysis, | 116 |
| abstract_inverted_index.atomistic | 120 |
| abstract_inverted_index.dedicated | 119 |
| abstract_inverted_index.evolution | 99 |
| abstract_inverted_index.formation | 180 |
| abstract_inverted_index.initially | 152 |
| abstract_inverted_index.knowledge | 62 |
| abstract_inverted_index.mechanism | 220 |
| abstract_inverted_index.plasmonic | 90 |
| abstract_inverted_index.promising | 76 |
| abstract_inverted_index.resulting | 177 |
| abstract_inverted_index.viewpoint | 210 |
| abstract_inverted_index.Bimetallic | 0 |
| abstract_inverted_index.Uncovering | 198 |
| abstract_inverted_index.attractive | 207 |
| abstract_inverted_index.bimetallic | 77 |
| abstract_inverted_index.biomedical | 12 |
| abstract_inverted_index.candidates | 5 |
| abstract_inverted_index.is\nhighly | 63 |
| abstract_inverted_index.microscopy | 131 |
| abstract_inverted_index.properties | 32 |
| abstract_inverted_index.structural | 124 |
| abstract_inverted_index.structure, | 39, 50 |
| abstract_inverted_index.synthesis. | 114 |
| abstract_inverted_index.tomography | 137 |
| abstract_inverted_index.we\nreport | 93 |
| abstract_inverted_index.a\ndetailed | 123 |
| abstract_inverted_index.crystalline | 102 |
| abstract_inverted_index.diffraction | 128 |
| abstract_inverted_index.properties, | 21 |
| abstract_inverted_index.resolution. | 146 |
| abstract_inverted_index.structures. | 197 |
| abstract_inverted_index.temperature | 170 |
| abstract_inverted_index.complemented | 117 |
| abstract_inverted_index.composition, | 37 |
| abstract_inverted_index.demonstrates | 192 |
| abstract_inverted_index.simulations, | 121 |
| abstract_inverted_index.Our\nin-depth | 115 |
| abstract_inverted_index.and\nmagnetic | 82 |
| abstract_inverted_index.applications, | 13 |
| abstract_inverted_index.body-centered | 189 |
| abstract_inverted_index.catalytically | 87 |
| abstract_inverted_index.compositions, | 163 |
| abstract_inverted_index.conditions.\n | 223 |
| abstract_inverted_index.counterparts. | 28 |
| abstract_inverted_index.metastability | 194 |
| abstract_inverted_index.nanoparticles | 1, 67 |
| abstract_inverted_index.phase,\nwhich | 191 |
| abstract_inverted_index.temperatures, | 58 |
| abstract_inverted_index.these\nunique | 199 |
| abstract_inverted_index.a\nfundamental | 209 |
| abstract_inverted_index.distributions, | 165 |
| abstract_inverted_index.nanostructures | 200 |
| abstract_inverted_index.ultrastructure | 184 |
| abstract_inverted_index.non-equilibrium | 222 |
| abstract_inverted_index.their\nchemical | 36 |
| abstract_inverted_index.characterization | 125 |
| abstract_inverted_index.crystallographic | 38 |
| abstract_inverted_index.of\ntechnological | 10 |
| abstract_inverted_index.their\nmonometallic | 27 |
| abstract_inverted_index.Au-Fe\nnanoparticles | 151 |
| abstract_inverted_index.catalytic,\noptical, | 18 |
| abstract_inverted_index.nanostructures\nwith | 158 |
| abstract_inverted_index.Au-Fe\nnanoparticles, | 105 |
| abstract_inverted_index.nanoscale,\ntransforms | 53 |
| abstract_inverted_index.transmission\nelectron | 130 |
| abstract_inverted_index.distribution.\nHowever, | 42 |
| abstract_inverted_index.nanoparticle\nformation | 219 |
| abstract_inverted_index.elemental\ndistributions | 140 |
| abstract_inverted_index.single\nface-centered-cubic | 183 |
| abstract_inverted_index.high-temperature\ncatalysis. | 72 |
| abstract_inverted_index.size-depended\nmicrostrains. | 167 |
| abstract_inverted_index.diffusion-controlled\nrecrystallization | 173 |
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| institutions_distinct_count | 12 |
| citation_normalized_percentile.value | 0.21218599 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |