Multiple Operando Fields Can Identify a Predictive Mass Transport Theory in Electrolytes Article Swipe
Aashutosh Mistry
,
Hans‐Georg Steinrück
,
Michael F. Toney
,
Nitash P. Balsara
,
Venkat Srinivasan
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpcc.4c06851
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpcc.4c06851
An electrolyte transport theory connects its transport properties, evolution of spatiotemporal fields (e.g., concentration), and corresponding macroscopic current and voltage responses. Given this interconnection, the transport properties are typically inferred by analyzing the macroscopic response through the lens of a chosen electrolyte transport theory. Unfortunately, the same macroscopic measurements can be analyzed by using different theories to arrive at seemingly dissimilar properties that are inconsistent with each other. We offer a resolution to this dilemma by analyzing multiple spatiotemporal (i.e., operando) fields for a given electrolyte. We show that predictive transport theory can analyze operando fields to estimate underlying transport properties and subsequently predict another operando field. A theory passing this test identifies meaningful transport properties such that the electrolyte behavior can be accurately predicted over a wide range of excitations, and is critical to property-based electrolyte screening and electrolyte discovery efforts.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.jpcc.4c06851
- OA Status
- gold
- Cited By
- 2
- References
- 97
- Related Works
- 10
- OpenAlex ID
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https://openalex.org/W4407020988Canonical identifier for this work in OpenAlex
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https://doi.org/10.1021/acs.jpcc.4c06851Digital Object Identifier
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Multiple Operando Fields Can Identify a Predictive Mass Transport Theory in ElectrolytesWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-01-31Full publication date if available
- Authors
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Aashutosh Mistry, Hans‐Georg Steinrück, Michael F. Toney, Nitash P. Balsara, Venkat SrinivasanList of authors in order
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https://doi.org/10.1021/acs.jpcc.4c06851Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://escholarship.org/uc/item/9503m0gmDirect OA link when available
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Electrolyte, Mass transport, Chemistry, Chemical engineering, Materials science, Environmental science, Computer science, Physics, Engineering physics, Engineering, Physical chemistry, ElectrodeTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2025: 2Per-year citation counts (last 5 years)
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