Nanoscale magnetism and magnetic phase transitions in atomically thin CrSBr Article Swipe

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Märta A. Tschudin , David A. Broadway , Patrick Reiser , Carolin Schrader , Evan J. Telford , B. Gross , Jordan M. Cox , Adrien E. E. Dubois , Daniel G. Chica , Ricardo Rama‐Eiroa , Elton J. G. Santos , Martino Poggio , Michael E. Ziebel , Cory R. Dean , Xavier Roy , Patrick Maletinsky ·

YOU? · · 2023 · Open Access · · DOI: https://doi.org/10.48550/arxiv.2312.09279

Since their first observation in 2017, atomically thin van der Waals (vdW) magnets have attracted significant fundamental, and application-driven attention. However, their low ordering temperatures, $T_c$, sensitivity to atmospheric conditions and difficulties in preparing clean large-area samples still present major limitations to further progress. The remarkably stable high-$T_c$ vdW magnet CrSBr has the potential to overcome these key shortcomings, but its nanoscale properties and rich magnetic phase diagram remain poorly understood. Here we use single spin magnetometry to quantitatively characterise saturation magnetization, magnetic anisotropy constants, and magnetic phase transitions in few-layer CrSBr by direct magnetic imaging. We show pristine magnetic phases, devoid of defects on micron length-scales, and demonstrate remarkable air-stability down the monolayer limit. We address the spin-flip transition in bilayer CrSBr by direct imaging of the emerging antiferromagnetic (AFM) to ferromagnetic (FM) phase wall and elucidate the magnetic properties of CrSBr around its ordering temperature. Our work will enable the engineering of exotic electronic and magnetic phases in CrSBr and the realisation of novel nanomagnetic devices based on this highly promising vdW magnet.

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Condensed Matter Physics

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Condensed matter physics Magnetism Materials science Antiferromagnetism Ferromagnetism Magnet Magnetization van der Waals force Spintronics Saturation (graph theory) Phase transition Magnetometer Magnetic anisotropy Nanotechnology Magnetic field Physics Combinatorics Mathematics Quantum mechanics Molecule

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Type: preprint
Language: en
Landing Page: http://arxiv.org/abs/2312.09279
PDF: https://arxiv.org/pdf/2312.09279
OA Status: green
Related Works: 10
OpenAlex ID: https://openalex.org/W4389911277

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DOI: https://doi.org/10.48550/arxiv.2312.09279

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Title: Nanoscale magnetism and magnetic phase transitions in atomically thin CrSBr

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Language: en

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Publication year: 2023

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Publication date: 2023-12-14

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Authors: Märta A. Tschudin, David A. Broadway, Patrick Reiser, Carolin Schrader, Evan J. Telford, B. Gross, Jordan M. Cox, Adrien E. E. Dubois, Daniel G. Chica, Ricardo Rama‐Eiroa, Elton J. G. Santos, Martino Poggio, Michael E. Ziebel, Cory R. Dean, Xavier Roy, Patrick Maletinsky

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Landing page: https://arxiv.org/abs/2312.09279

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Concepts: Condensed matter physics, Magnetism, Materials science, Antiferromagnetism, Ferromagnetism, Magnet, Magnetization, van der Waals force, Spintronics, Saturation (graph theory), Phase transition, Magnetometer, Magnetic anisotropy, Nanotechnology, Magnetic field, Physics, Combinatorics, Mathematics, Quantum mechanics, Molecule

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