Natural magmatic granite as matrix for immobilizing simulated An4+ waste Article Swipe
Lingshuang Li
,
Xiaoyan Shu
,
Hexi Tang
,
Shunzhang Chen
,
Wenxiao Huang
,
Guilin Wei
,
Dadong Shao
,
Yi Xie
,
Xirui Lu
·
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-23879/v1
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-23879/v1
In nature, many rocks contain radionuclides, and returning radioactive waste to nature is an environmentally friendly way. In this work, a natural magmatic granite rock has been studied as a host matrix for simulated An 4+ waste disposal. The blank granite, in the form of powder, was firstly treated by muffle furnace heating in the temperature range of 800 °C to 1400 °C. It was found that the lowest crystallinity of the samples was obtained at 1300 °C. Moreover, 8 wt .% of simulated tetravalent actinides (CeO 2 ) could be successfully immobilized in the natural granite at 1300 °C for 60 min. Raman results show the structure disordering in samples tends to increase with the increased amount of CeO 2 . SEM-EDS observation shows that the distribution of Ce was relatively uniform in the matrix. Moreover, the hardness of solidified body is comparable to traditional glasses and it decreases with the increase of CeO 2 content.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-23879/v1
- OA Status
- green
- Related Works
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- OpenAlex ID
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https://doi.org/10.21203/rs.3.rs-23879/v1Digital Object Identifier
- Title
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Natural magmatic granite as matrix for immobilizing simulated An4+ wasteWork title
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preprintOpenAlex work type
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enPrimary language
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2020Year of publication
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2020-04-23Full publication date if available
- Authors
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Lingshuang Li, Xiaoyan Shu, Hexi Tang, Shunzhang Chen, Wenxiao Huang, Guilin Wei, Dadong Shao, Yi Xie, Xirui LuList of authors in order
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-
https://doi.org/10.21203/rs.3.rs-23879/v1Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
- OA URL
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https://doi.org/10.21203/rs.3.rs-23879/v1Direct OA link when available
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Natural (archaeology), Geochemistry, Geology, Matrix (chemical analysis), Waste management, Environmental science, Mining engineering, Chemistry, Engineering, Paleontology, ChromatographyTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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