No Evidence of Benefits of Host Nano-Carbon Materials for Practical Lithium Anode-Free Cells Article Swipe

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Bingxin Zhou , Baizeng Fang , Ivan Stoševski , Arman Bonakdarpour , David P. Wilkinson ·

YOU? · · 2022 · Open Access · · DOI: https://doi.org/10.3390/nano12091413

Nano-carbon-based materials are widely reported as lithium host materials in lithium metal batteries (LMBs); however, researchers report contradictory claims as to where the lithium plating occurs. Herein, the use of pure hollow core-carbon spheres coated on Cu (PHCCSs@Cu) to study the lithium deposition behavior with respect to this type of structure in lithium anode-free cells is described. It is demonstrated that the lithium showed some initial and limited intercalation into the PHCCSs and then plated on the external carbon walls and the top surface of the carbon coating during the charging process. The unfavorable deposition of lithium inside the PHCCSs is discussed from the viewpoint of lithium-ion transport and lithium nucleation. The application potential of PHCCSs and the data from these LMB studies are also discussed.

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Intercalation (Chemistry)

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Lithium (medication) Anode Materials science Carbon fibers Lithium metal Nucleation Coating Nanotechnology Deposition (geology) Intercalation (chemistry) Chemical engineering Inorganic chemistry Composite material Chemistry Composite number Electrode Medicine Biology Engineering Endocrinology Physical chemistry Organic chemistry Sediment Paleontology

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Type: article
Language: en
Landing Page: https://doi.org/10.3390/nano12091413
PDF: https://www.mdpi.com/2079-4991/12/9/1413/pdf?version=1650522332
OA Status: gold
Cited By: 5
References: 35
Related Works: 10
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DOI: https://doi.org/10.3390/nano12091413

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Title: No Evidence of Benefits of Host Nano-Carbon Materials for Practical Lithium Anode-Free Cells

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Language: en

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Publication year: 2022

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Publication date: 2022-04-20

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Authors: Bingxin Zhou, Baizeng Fang, Ivan Stoševski, Arman Bonakdarpour, David P. Wilkinson

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Landing page: https://doi.org/10.3390/nano12091413

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Concepts: Lithium (medication), Anode, Materials science, Carbon fibers, Lithium metal, Nucleation, Coating, Nanotechnology, Deposition (geology), Intercalation (chemistry), Chemical engineering, Inorganic chemistry, Composite material, Chemistry, Composite number, Electrode, Medicine, Biology, Engineering, Endocrinology, Physical chemistry, Organic chemistry, Sediment, Paleontology

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Cited by: 5

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