On the stability of neon cluster ions – Evidence for isomeric structures Article Swipe
Siegfried Kollotzek
,
Stefan Bergmeister
,
Lukas Tiefenthaler
,
Simon Albertini
,
Elisabeth Gruber
,
Fábio Zappa
,
P. Scheier
,
O. Echt
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1016/j.ijms.2021.116528
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1016/j.ijms.2021.116528
We have adopted the newly developed technique of growing cationic clusters in size-to-charge selected helium nanodroplets (HNDs), with subsequent removal of helium in a collision cell, to record high-resolution mass spectra of Nen+. Growth in singly charged HNDs leads to mass spectra that feature the same anomalies in the cluster ion abundance as in previous work, namely maxima at n = 14, 21, 55/56, 75. Several other, weaker but statistically significant anomalies are observed at n = 9, 26, 29, 33, 35, 69, 82, 89. However, when neon clusters are grown in larger HNDs, which are likely to be multiply charged, we observe a different set of magic numbers, at n = 7, 13, 19, 26, 29, 34, 55, 71, 81, plus many other numbers for larger clusters, up to n = 197. A transition from the first to the second set is observed in a limited size range if the collision pressure is increased. The most likely reason for the existence of two different sets of magic numbers appears to be the existence of two distinct structural families.
Related Topics
Concepts
Chemistry
Neon
Ion
Cluster (spacecraft)
Spectral line
Magic number (chemistry)
Helium
Atomic physics
Mass spectrum
Cluster size
Analytical Chemistry (journal)
Molecular dynamics
Physics
Computational chemistry
Electronic structure
Chromatography
Organic chemistry
Programming language
Argon
Computer science
Astronomy
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.ijms.2021.116528
- OA Status
- hybrid
- Cited By
- 2
- References
- 112
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3124060997
All OpenAlex metadata
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https://openalex.org/W3124060997Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.ijms.2021.116528Digital Object Identifier
- Title
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On the stability of neon cluster ions – Evidence for isomeric structuresWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-01-23Full publication date if available
- Authors
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Siegfried Kollotzek, Stefan Bergmeister, Lukas Tiefenthaler, Simon Albertini, Elisabeth Gruber, Fábio Zappa, P. Scheier, O. EchtList of authors in order
- Landing page
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https://doi.org/10.1016/j.ijms.2021.116528Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://doi.org/10.1016/j.ijms.2021.116528Direct OA link when available
- Concepts
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Chemistry, Neon, Ion, Cluster (spacecraft), Spectral line, Magic number (chemistry), Helium, Atomic physics, Mass spectrum, Cluster size, Analytical Chemistry (journal), Molecular dynamics, Physics, Computational chemistry, Electronic structure, Chromatography, Organic chemistry, Programming language, Argon, Computer science, AstronomyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
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2022: 1, 2021: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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