Optimized thermoelectric performance driven by A-site deficient in SrxLa0.1TiO3/Ti composites Article Swipe
Zhihao Lou
,
Ping Zhang
,
Penghui Chen
,
Ziyao Wei
,
Jian‐Jun Gou
,
Jie Xu
,
Chunlin Gong
,
Feng Gao
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-2959967/v1
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-2959967/v1
For thermoelectric applications at high temperatures, perovskite SrTiO 3 is a promising contender as an n-type oxide thermoelectric (TE) material. In this work, Sr x La 0.1 TiO 3 /Ti composite ceramics were successfully synthesized by solid state reaction with a combination of the A-site cation vacancy and fabricating composite. Through XRD and SEM analysis, a complex microstructure composed of two kinds of titanium oxides was formed after reductive sintering and annealing. In addition, controlling the content of Sr vacancies in the Sr x La 0.1 TiO 3 matrix increased the thermoelectric power factor by optimizing the weighted mobility in the composite, resulting in the highest power factor PF of 425.8 µWm − 1 K − 2 and the maximum ZT of 0.16 for the Sr 0.875 La 0.1 TiO 3 /Ti composite through the synergistic optimization of electrical and thermal transport properties. The strategy proposed in this study of design A-site-deficient composites with nano-sized metal paved a new way to fabricate high performance oxide thermoelectric materials.
Related Topics
Concepts
Thermoelectric effect
Materials science
Composite number
Microstructure
Sintering
Annealing (glass)
Oxide
Thermoelectric materials
Composite material
Seebeck coefficient
Thermoelectric generator
Perovskite (structure)
Ceramic
Chemical engineering
Metallurgy
Thermal conductivity
Physics
Engineering
Thermodynamics
Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-2959967/v1
- https://www.researchsquare.com/article/rs-2959967/latest.pdf
- OA Status
- green
- References
- 41
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4378211580
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4378211580Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.21203/rs.3.rs-2959967/v1Digital Object Identifier
- Title
-
Optimized thermoelectric performance driven by A-site deficient in SrxLa0.1TiO3/Ti compositesWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-05-25Full publication date if available
- Authors
-
Zhihao Lou, Ping Zhang, Penghui Chen, Ziyao Wei, Jian‐Jun Gou, Jie Xu, Chunlin Gong, Feng GaoList of authors in order
- Landing page
-
https://doi.org/10.21203/rs.3.rs-2959967/v1Publisher landing page
- PDF URL
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https://www.researchsquare.com/article/rs-2959967/latest.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
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https://www.researchsquare.com/article/rs-2959967/latest.pdfDirect OA link when available
- Concepts
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Thermoelectric effect, Materials science, Composite number, Microstructure, Sintering, Annealing (glass), Oxide, Thermoelectric materials, Composite material, Seebeck coefficient, Thermoelectric generator, Perovskite (structure), Ceramic, Chemical engineering, Metallurgy, Thermal conductivity, Physics, Engineering, ThermodynamicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- References (count)
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41Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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