Origin of relaxor behavior in barium titanate based lead-free relaxors Article Swipe
Vignaswaran K. Veerapandiyan
,
Maxim N. Popov
,
Florian Mayer
,
Jürgen Spitaler
,
Šarūnas Svirskas
,
Vidmantas Kalendra
,
Jonas Lins
,
Giovanna Canu
,
María Teresa Buscaglia
,
Marek Paściak
,
J. Banys
,
Pedro B. Groszewicz
,
Vincenzo Buscaglia
,
J. Hlinka
,
Marco Deluca
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.5281/zenodo.5642828
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.5281/zenodo.5642828
It is well known that disordered relaxor ferroelectrics exhibit local polar correlations. The origin of localized fields that disrupt long range polar order for different substitution types, however, is unclear. Currently, it is known that substituents of the same valence as Ti4+ at the B-site of barium titanate lattice produce random disruption of Ti-O-Ti chains that induces relaxor behavior. On the other hand, investigating lattice disruption and relaxor behavior resulting from substituents of different valence at the B-site is more complex due to the simultaneous occurrence of charge imbalances and displacements of the substituent cation. The existence of an effective charge mediated mechanism for relaxor behavior appearing at low (<10%) substituent contents in heterovalent modified barium titanate ceramics is evinced from this data, which underpin the publication by the same name currently in press by Advanced Electronic Materials. These results will add credits to the current understanding of relaxor behavior in chemically modified ferroelectric materials and also acknowledge the critical role of defects (such as cation vacancies) in lattice disruption, paving the way for chemistry-based materials design in the field of dielectric and energy storage applications
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- Type
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- en
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- OA Status
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- Related Works
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https://doi.org/10.5281/zenodo.5642828Digital Object Identifier
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Origin of relaxor behavior in barium titanate based lead-free relaxorsWork title
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datasetOpenAlex work type
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enPrimary language
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2021Year of publication
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2021-01-01Full publication date if available
- Authors
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Vignaswaran K. Veerapandiyan, Maxim N. Popov, Florian Mayer, Jürgen Spitaler, Šarūnas Svirskas, Vidmantas Kalendra, Jonas Lins, Giovanna Canu, María Teresa Buscaglia, Marek Paściak, J. Banys, Pedro B. Groszewicz, Vincenzo Buscaglia, J. Hlinka, Marco DelucaList of authors in order
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://doi.org/10.5281/zenodo.5642828Direct OA link when available
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Barium titanate, Barium, Materials science, Lead (geology), Mineralogy, Chemistry, Composite material, Metallurgy, Ceramic, Geology, GeomorphologyTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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