Parallel-mode EPR spectra of the hexaaqua manganese(II) Ion in tetrahedral symmetry Article Swipe
Margrete Juel Henrichsen
,
Jesper Bendix
,
Høgni Weihe
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.5802/crchim.266
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.5802/crchim.266
Parallel-mode X-band EPR spectra of the manganese(II) hexaaqua ion as substitutional impurity in Cs[Mg(H 2 O) 6 ]AsO 4 are presented and interpreted. In this lattice the aqua ion, considering also the disposition of the hydrogen atoms, occupies a crystallographic site with tetrahedral symmetry. This rare situation enables that the line positions as well as the intensities in the parallel-mode EPR spectra can be modelled with a simple three-parameter cubic-symmetry spin Hamiltonian, including the isotropic Zeeman interaction ( ) pertinent to the electronic spin, the isotropic hyperfine interaction ( ), between the electronic spin and the nuclear spin, and the cubic splitting ( ) of the manifold. A simple formalism, based on perturbation theory to grossly account for the observed intensities, is presented. We observe all parallel-mode-allowed hyperfine transitions associated with all fine-structure transitions.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.5802/crchim.266
- https://comptes-rendus.academie-sciences.fr/chimie/item/10.5802/crchim.266.pdf
- OA Status
- diamond
- Cited By
- 1
- References
- 24
- Related Works
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- OpenAlex ID
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https://doi.org/10.5802/crchim.266Digital Object Identifier
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Parallel-mode EPR spectra of the hexaaqua manganese(II) Ion in tetrahedral symmetryWork title
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articleOpenAlex work type
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enPrimary language
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2024Year of publication
- Publication date
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2024-02-12Full publication date if available
- Authors
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Margrete Juel Henrichsen, Jesper Bendix, Høgni WeiheList of authors in order
- Landing page
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https://doi.org/10.5802/crchim.266Publisher landing page
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https://comptes-rendus.academie-sciences.fr/chimie/item/10.5802/crchim.266.pdfDirect link to full text PDF
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YesWhether a free full text is available
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diamondOpen access status per OpenAlex
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https://comptes-rendus.academie-sciences.fr/chimie/item/10.5802/crchim.266.pdfDirect OA link when available
- Concepts
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Manganese, Tetrahedron, Electron paramagnetic resonance, Tetrahedral symmetry, Ion, Symmetry (geometry), Chemistry, Spectral line, Crystallography, Nuclear magnetic resonance, Physics, Geometry, Organic chemistry, Quantum mechanics, Rotational symmetry, Mathematics, MechanicsTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2025: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W2060986410, https://openalex.org/W1966006736, https://openalex.org/W2077272804, https://openalex.org/W2145200107, https://openalex.org/W4234961905, https://openalex.org/W1980079008, https://openalex.org/W4285391409, https://openalex.org/W3084865288, https://openalex.org/W2081804488, https://openalex.org/W2018417075, https://openalex.org/W6678806270, https://openalex.org/W2124867702, https://openalex.org/W2081221613, https://openalex.org/W1986014945, https://openalex.org/W2005047466, https://openalex.org/W1991308198, https://openalex.org/W2007757199, https://openalex.org/W2082776444, https://openalex.org/W1994071819, https://openalex.org/W2083267348, https://openalex.org/W2074556456, https://openalex.org/W248369785, https://openalex.org/W2124464977, https://openalex.org/W1510913788 |
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