Phase-matching of high harmonic generation in twisted solids Article Swipe
Chenjun Ma
,
Chen Huang
,
Yilong You
,
Huazhan Liu
,
Zijing Ding
,
Mengxian Ding
,
Jin Zhang
,
Guixin Li
,
Z. Sun
,
Shiwei Wu
,
Chaojie Ma
,
Enge Wang
,
Hong Hao
,
Kaihui Liu
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2503.08052
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2503.08052
High harmonic generation (HHG) in solids could enable attosecond and ultraviolet light sources with high compactness, great controllability and rich functions. However, the HHG process is accompanied by a quite large wavevector mismatch that is uncompensated by any traditional phase-matching method, directly limiting its energy conversion efficiency. Here, we propose an effective strategy for phase-matching of HHG with arbitrary harmonic orders in solids. Two flakes of solids with an interlayer twist induce a nonlinear optical phase that depends on the crystal symmetry, twist angle and harmonic order, which can be accurately designed to compensate for the phase mismatch in HHG. Guided by the twist-phase-matching theory, we achieved a record-high conversion efficiency of $~1.5\times10^{-5}$ for the fifth HHG in twisted hexagonal boron nitride crystals with a total thickness of only 1 $μm$. Our work establishes a foundation for developing ultrashort-wavelength and ultrafast-pulse laser sources in compact solid-state tabletop systems for fundamental and applied sciences.
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- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2503.08052
- https://arxiv.org/pdf/2503.08052
- OA Status
- green
- OpenAlex ID
- https://openalex.org/W4414567945
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https://openalex.org/W4414567945Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2503.08052Digital Object Identifier
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Phase-matching of high harmonic generation in twisted solidsWork title
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preprintOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-03-11Full publication date if available
- Authors
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Chenjun Ma, Chen Huang, Yilong You, Huazhan Liu, Zijing Ding, Mengxian Ding, Jin Zhang, Guixin Li, Z. Sun, Shiwei Wu, Chaojie Ma, Enge Wang, Hong Hao, Kaihui LiuList of authors in order
- Landing page
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https://arxiv.org/abs/2503.08052Publisher landing page
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https://arxiv.org/pdf/2503.08052Direct link to full text PDF
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://arxiv.org/pdf/2503.08052Direct OA link when available
- Cited by
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0Total citation count in OpenAlex
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