Phosphorus removal from aqueous solution by adsorption using wetland-based biochar: Batch experiment Article Swipe
QiaoLing Xu
,
Li Wang
,
Minxia Tan
,
Xiaolei Wang
,
Jiajie Li
,
Hejun Geng
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1515/gps-2022-0046
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1515/gps-2022-0046
This article experiments wetland-based biochar as an effective adsorbent for phosphorus removal. In this experiment, four common wetland plants, canna (C), umbrella palm (U), bamboo reed (B), and Thalia dealbata (T), were used as the main raw materials. Twelve kinds of biochar (C300, C500, C700, U300, U500, U700, B300, B500, B700, T300, T500, and T700) were obtained at three pyrolysis temperatures (300°C, 500°C, and 700°C). The results show that canna (C) and umbrella palm (U) are more suitable as raw materials for phosphorus removal using biochar. If bamboo reed (B) and Thalia dealbata (T) are used as raw materials for phosphorus removal using biochar, there is a greater risk of phosphorus release. With the increase of pyrolysis temperature (700°C > 500°C > 300°C), there is an increasing trend of phosphorus adsorption effect. The theoretical maximum adsorption capacity of C700, U700, and C500 was 39.24, 7.08, and 7.26 mg P·g −1 at an initial concentration of 50 mg·L −1 phosphorus, respectively. The theoretical adsorption capacity of C700 ( Q max = 39.24 mg P·g −1 ) was much higher than that of the general modified adsorption materials. It also has a larger tolerance range to pH (3–11). The results of kinetic model fitting showed that the adsorption mechanism of C700, U700, and C500 on phosphorus can be better simulated by intra-particle diffusion and Elovich model, and the adsorption mechanism includes surface adsorption and intra-particle diffusion. The fitting of isothermal adsorption model showed that Langmuir–Freundlich equation is more suitable for the description of adsorption characteristics of C700, U700, and C500, and the fitting coefficient R 2 is 0.9928, 0.9949, and 0.9897, respectively. It indicates that the adsorption of phosphorus on C700, U700, and C500 has a balance of uniform and nonuniform surface, and monolayer and multilayer adsorption could occur. The results from this work demonstrated that the biochar obtained from canna at 700°C has good adsorption and phosphorus removal potential without modification, and it can be used as the preferred biochar for phosphorus removal of high concentration with large pH changes. In the final validation experiment, the phosphorus removal rate of C700 was up to 77.4% on the treatment of actual phosphorus containing wastewater.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1515/gps-2022-0046
- https://www.degruyter.com/document/doi/10.1515/gps-2022-0046/pdf
- OA Status
- gold
- Cited By
- 10
- References
- 17
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4285277918
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4285277918Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1515/gps-2022-0046Digital Object Identifier
- Title
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Phosphorus removal from aqueous solution by adsorption using wetland-based biochar: Batch experimentWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-01-01Full publication date if available
- Authors
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QiaoLing Xu, Li Wang, Minxia Tan, Xiaolei Wang, Jiajie Li, Hejun GengList of authors in order
- Landing page
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https://doi.org/10.1515/gps-2022-0046Publisher landing page
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https://www.degruyter.com/document/doi/10.1515/gps-2022-0046/pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.degruyter.com/document/doi/10.1515/gps-2022-0046/pdfDirect OA link when available
- Concepts
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Biochar, Adsorption, Phosphorus, Pyrolysis, Aqueous solution, Chemistry, Diffusion, Chemical engineering, Pulp and paper industry, Nuclear chemistry, Environmental chemistry, Organic chemistry, Thermodynamics, Physics, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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10Total citation count in OpenAlex
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2025: 2, 2024: 6, 2023: 2Per-year citation counts (last 5 years)
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17Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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