Photo‐ and Electrochemical Properties of a CO2 Reducing Ruthenium–Rhenium Quaterpyridine‐Based Catalyst Article Swipe
Liam Frayne
,
Nivedita Das
,
Avishek Paul
,
Saeed Amirjalayer
,
Wybren Jan Buma
,
Sander Woutersen
,
Conor Long
,
Johannes G. Vos
,
Mary T. Pryce
·
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.1002/cptc.201700197
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.1002/cptc.201700197
The bridging ligand 2,2′,5′,3′′,6′′,2′′′‐quaterpyridine was utilised to tether [(bpy) 2 Ru] 2+ and [Re(CO) 3 Cl] subunits for the purpose of photocatalytic CO 2 reduction. The photophysics and electrochemistry of the complex and associated mononuclear species are reported herein, in addition to photocatalytic, picosecond time‐resolved infrared and computational studies. Photophysical, time‐resolved IR, and electrochemical data together with quantum chemical calculations indicate weak communication between the two metal centres. As a result of the electron‐withdrawing effect of the ligand on both the Ru and Re subunits, the reducing power of the photosensitiser and catalytic unit were significantly attenuated relative to the intermolecular approach utilising [(bpy) 3 Ru] 2+ and (bpy)Re(CO) 3 Cl.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/cptc.201700197
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cptc.201700197
- OA Status
- bronze
- Cited By
- 27
- References
- 78
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2792763139
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- OpenAlex ID
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https://openalex.org/W2792763139Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/cptc.201700197Digital Object Identifier
- Title
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Photo‐ and Electrochemical Properties of a CO2 Reducing Ruthenium–Rhenium Quaterpyridine‐Based CatalystWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2018Year of publication
- Publication date
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2018-02-15Full publication date if available
- Authors
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Liam Frayne, Nivedita Das, Avishek Paul, Saeed Amirjalayer, Wybren Jan Buma, Sander Woutersen, Conor Long, Johannes G. Vos, Mary T. PryceList of authors in order
- Landing page
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https://doi.org/10.1002/cptc.201700197Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cptc.201700197Direct link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cptc.201700197Direct OA link when available
- Concepts
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Rhenium, Ruthenium, Electrochemistry, Catalysis, Picosecond, Photochemistry, Ligand (biochemistry), Photocatalysis, Bridging ligand, Chemistry, Intermolecular force, Infrared, Metal, Inorganic chemistry, Molecule, Physical chemistry, Electrode, Organic chemistry, Biochemistry, Optics, Laser, Receptor, PhysicsTop concepts (fields/topics) attached by OpenAlex
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27Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 6, 2023: 4, 2022: 2, 2021: 3Per-year citation counts (last 5 years)
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78Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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