Photoluminescence Modulation of Graphene/MoS2 Heterostructures Separated by Laser-Induced Functionalization Article Swipe
Qing Cao
,
Mira Kreßler
,
Marleen Hußmann
,
Yalei Hu
,
Patryk Kusch
,
Siegfried Eigler
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1021/acs.chemmater.3c03166
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1021/acs.chemmater.3c03166
Tuning the optoelectronic properties of monolayer MoS2 (1L-MoS2) is highly desired for optoelectronic applications. Gaining profound insights into the fundamental mechanisms that govern optoelectronic properties is of utmost significance. Here, we demonstrate that the photoluminescence (PL) of 1L-MoS2 can be modulated by photochemically functionalized graphene (F-G), which is covalently modified by oligophenyl groups. More importantly, the layer stacking sequence of F-G and 1L-MoS2 brings different interface structures, resulting in a significant difference in the PL enhancement. MoS2 supported by F-G (F-G/MoS2) has a 5-fold PL enhancement, while it only shows a 1.8-fold PL enhancement if stacked underneath F-G (MoS2/F-G). Accordingly, the results indicate that the oligophenyl groups in F-G/MoS2 not only have a p-doping effect on MoS2 but also largely prevent electron donation from the graphene basal plane with an enlarged interlayer distance of 8 nm. Consequently, the PL enhancement is lost with the thermal defunctionalization of F-G. Thus, we conclude that the functional groups can be considered as separate molecular components with the vertical arrangement in the functionalized heterostructure system. The photoactive graphene acts as a template for perpendicular molecular alignment in the heterointerface construction. The F-G/MoS2 heterostructures bring new perspectives to the design and investigation of optoelectronic devices.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.chemmater.3c03166
- OA Status
- hybrid
- Cited By
- 7
- References
- 39
- Related Works
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- OpenAlex ID
- https://openalex.org/W4391873919
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4391873919Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.chemmater.3c03166Digital Object Identifier
- Title
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Photoluminescence Modulation of Graphene/MoS2 Heterostructures Separated by Laser-Induced FunctionalizationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-02-16Full publication date if available
- Authors
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Qing Cao, Mira Kreßler, Marleen Hußmann, Yalei Hu, Patryk Kusch, Siegfried EiglerList of authors in order
- Landing page
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https://doi.org/10.1021/acs.chemmater.3c03166Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://doi.org/10.1021/acs.chemmater.3c03166Direct OA link when available
- Concepts
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Surface modification, Graphene, Photoluminescence, Heterojunction, Materials science, Modulation (music), Laser, Optoelectronics, Nanotechnology, Chemistry, Optics, Physics, Physical chemistry, AcousticsTop concepts (fields/topics) attached by OpenAlex
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7Total citation count in OpenAlex
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2025: 4, 2024: 3Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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