Plasma-Catalytic CO2 Reforming of Toluene over Hydrotalcite-Derived NiFe/(Mg, Al)Ox Catalysts Article Swipe
Lina Liu
,
Jing Dai
,
Sonali Das
,
Yaolin Wang
,
Han Yu
,
Shibo Xi
,
Zhikun Zhang
,
Xin Tu
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/jacsau.2c00603
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1021/jacsau.2c00603
The removal of tar and CO2 in syngas from biomass gasification is crucial for the upgrading and utilization of syngas. CO2 reforming of tar (CRT) is a potential solution which simultaneously converts the undesirable tar and CO2 to syngas. In this study, a hybrid dielectric barrier discharge (DBD) plasma-catalytic system was developed for the CO2 reforming of toluene, a model tar compound, at a low temperature (∼200 °C) and ambient pressure. Periclase-phase (Mg, Al)O x nanosheet-supported NiFe alloy catalysts with various Ni/Fe ratios were synthesized from ultrathin Ni-Fe-Mg-Al hydrotalcite precursors and employed in the plasma-catalytic CRT reaction. The result demonstrated that the plasma-catalytic system is promising in promoting the low-temperature CRT reaction by generating synergy between DBD plasma and the catalyst. Among the various catalysts, Ni4Fe1-R exhibited superior activity and stability because of its highest specific surface area, which not only provided sufficient active sites for the adsorption of reactants and intermediates but also enhanced the electric field in the plasma. Furthermore, the stronger lattice distortion of Ni4Fe1-R provided more isolated O2- for CO2 adsorption, and having the most intensive interaction between Ni and Fe in Ni4Fe1-R restrained the catalyst deactivation induced by the segregation of Fe from the alloy to form FeO x . Finally, in situ Fourier transform infrared spectroscopy combined with comprehensive catalyst characterization was used to elucidate the reaction mechanism of the plasma-catalytic CRT reaction and gain new insights into the plasma-catalyst interfacial effect.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/jacsau.2c00603
- https://pubs.acs.org/doi/pdf/10.1021/jacsau.2c00603
- OA Status
- gold
- Cited By
- 44
- References
- 63
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4321204528
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4321204528Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/jacsau.2c00603Digital Object Identifier
- Title
-
Plasma-Catalytic CO2 Reforming of Toluene over Hydrotalcite-Derived NiFe/(Mg, Al)Ox CatalystsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-02-17Full publication date if available
- Authors
-
Lina Liu, Jing Dai, Sonali Das, Yaolin Wang, Han Yu, Shibo Xi, Zhikun Zhang, Xin TuList of authors in order
- Landing page
-
https://doi.org/10.1021/jacsau.2c00603Publisher landing page
- PDF URL
-
https://pubs.acs.org/doi/pdf/10.1021/jacsau.2c00603Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://pubs.acs.org/doi/pdf/10.1021/jacsau.2c00603Direct OA link when available
- Concepts
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Catalysis, Syngas, Hydrotalcite, Bimetallic strip, Materials science, Chemical engineering, Dielectric barrier discharge, Inorganic chemistry, Chemistry, Organic chemistry, Dielectric, Engineering, OptoelectronicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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44Total citation count in OpenAlex
- Citations by year (recent)
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2025: 20, 2024: 17, 2023: 7Per-year citation counts (last 5 years)
- References (count)
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63Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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