Plasma‐Enabled Process with Single‐Atom Catalysts for Sustainable Plastic Waste Transformation Article Swipe
Xiao Yu
,
Zhiqiang Rao
,
Guoxing Chen
,
Yuantao Yang
,
Songhak Yoon
,
Lina Liu
,
Zeai Huang
,
Marc Widenmeyer
,
Heng Guo
,
Gert Homm
,
Ulrike Kunz
,
Xingmin Liu
,
Emanuel Ionescu
,
Leopoldo Molina‐Luna
,
Xin Tu
,
Ying Zhou
,
Anke Weidenkaff
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202404196
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202404196
The escalating issue of plastic waste generation has prompted the search for an effective solution to address these challenges. In this study, we present a novel plasma‐enabled strategy for the rapid breakdown of various types of plastic wastes, including mixtures, into high‐value carbon nanomaterials and hydrogen. The H 2 yield and selectivity achieved through the implemented catalyst‐free plasma‐enabled strategy are 14.2 and 5.9 times higher, respectively, compared to those obtained with conventional thermal pyrolysis under similar conditions. It is noteworthy that this catalyst‐free plasma alone approach yields a significantly higher energy yield of H 2 (g H2 /kWh) compared to other pyrolysis processes. By coupling plasma pyrolysis with thermal catalytic process, employing of 1 wt . % M /CeO 2 ( M =Fe, Co, and Ni) atomically dispersed catalysts can further enhance hydrogen production. Specifically, the 1 wt . % Co/CeO 2 catalyst demonstrated excellent catalytic performance throughout the 10 cycles of plastic waste decomposition, achieving the highest H 2 yield of 46.7 mmol/g plastic (equivalent to 64.4 % of theoretical H 2 production) and nearly 100 % hydrogen atom recovery efficiency at the 7 th cycle. Notably, the H 2 yield achieved over the atomically dispersed Fe on CeO 2 surface (1 wt . % Fe/CeO 2 ) in the integrated plasma‐thermal catalytic process is comparable to that obtained with Fe particles on CeO 2 surface (10 wt . % Fe/CeO 2 ). This outcome, demonstrated with single‐atom catalysts, offers a promising avenue for cost‐effective and efficient chemical plastic recycling. Through a combination of experimental and computational efforts, we have provided an in‐depth understanding of the catalytic mechanisms of the investigated single atom catalysts in the developed plasma‐enabled process. This innovative and straightforward approach provides a promising and expedient strategy for continuously converting diverse plastic waste streams, including mixed and contaminated sources, into high‐value products conducive to a circular plastic economy.
Related Topics
Concepts
Catalysis
Materials science
Yield (engineering)
Pyrolysis
Chemical engineering
Hydrogen
Thermal decomposition
Decomposition
Heat of combustion
Hydrogen production
Plasma
Carbon fibers
Nanomaterials
Waste management
Nanotechnology
Organic chemistry
Chemistry
Metallurgy
Composite material
Combustion
Composite number
Engineering
Quantum mechanics
Physics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/anie.202404196
- OA Status
- green
- Cited By
- 15
- References
- 47
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4401715803
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4401715803Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/anie.202404196Digital Object Identifier
- Title
-
Plasma‐Enabled Process with Single‐Atom Catalysts for Sustainable Plastic Waste TransformationWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-08-20Full publication date if available
- Authors
-
Xiao Yu, Zhiqiang Rao, Guoxing Chen, Yuantao Yang, Songhak Yoon, Lina Liu, Zeai Huang, Marc Widenmeyer, Heng Guo, Gert Homm, Ulrike Kunz, Xingmin Liu, Emanuel Ionescu, Leopoldo Molina‐Luna, Xin Tu, Ying Zhou, Anke WeidenkaffList of authors in order
- Landing page
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https://doi.org/10.1002/anie.202404196Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
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https://www.ncbi.nlm.nih.gov/pmc/articles/11610705Direct OA link when available
- Concepts
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Catalysis, Materials science, Yield (engineering), Pyrolysis, Chemical engineering, Hydrogen, Thermal decomposition, Decomposition, Heat of combustion, Hydrogen production, Plasma, Carbon fibers, Nanomaterials, Waste management, Nanotechnology, Organic chemistry, Chemistry, Metallurgy, Composite material, Combustion, Composite number, Engineering, Quantum mechanics, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
15Total citation count in OpenAlex
- Citations by year (recent)
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2025: 14, 2024: 1Per-year citation counts (last 5 years)
- References (count)
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47Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W4322154573, https://openalex.org/W4285807626, https://openalex.org/W3205777154, https://openalex.org/W3012481340, https://openalex.org/W3161506990, https://openalex.org/W4385469048, https://openalex.org/W4383163093, https://openalex.org/W4220976445, https://openalex.org/W4206162572, https://openalex.org/W4319460918, https://openalex.org/W4225726171, https://openalex.org/W3215371806, https://openalex.org/W4312161555, https://openalex.org/W3092088280, https://openalex.org/W3014944207, https://openalex.org/W4206407072, https://openalex.org/W4321378445, https://openalex.org/W4387536761, https://openalex.org/W3082009060, https://openalex.org/W4323306096, https://openalex.org/W4224293850, https://openalex.org/W4319872637, https://openalex.org/W3094916216, https://openalex.org/W4224304957, https://openalex.org/W4285500512, https://openalex.org/W4324342777, https://openalex.org/W3184608709, https://openalex.org/W3183641110, https://openalex.org/W3002230200, https://openalex.org/W2973839888, https://openalex.org/W4292985552, https://openalex.org/W4367671643, https://openalex.org/W1991914316, https://openalex.org/W4387191231, https://openalex.org/W2024914119, https://openalex.org/W2235679284, https://openalex.org/W2019011995, https://openalex.org/W2038754799, https://openalex.org/W2527498606, https://openalex.org/W3094410550, https://openalex.org/W3162362376, https://openalex.org/W4283264143, https://openalex.org/W2886718281, https://openalex.org/W2802243083, https://openalex.org/W3086254212, https://openalex.org/W4401715803, https://openalex.org/W4206934262 |
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