Polyamorphism of vapor-deposited amorphous selenium in response to light Article Swipe
Aixi Zhang
,
Yi Jin
,
Tianyi Liu
,
R. B. Stephens
,
Zahra Fakhraai
·
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1073/pnas.2009852117
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1073/pnas.2009852117
Significance Amorphous selenium (a-Se) has a complicated molecular structure with overcoordinated defects and dangling bonds. This light-sensitive structure can undergo significant changes including bond breakage, reconnection, and defect formation upon illumination with above-bandgap light. Light sensitivity makes a-Se a unique system to study the role of surface structure and dynamics on stable glass formation during physical vapor deposition. We show that illumination during deposition produces less dense, more anisotropic, and kinetically more stable glasses, due to better network formation at the surface. This is a demonstration that light can be used to manipulate surface properties to generate distinct polyamorphic solid states that are not accessible through liquid quenching or aging.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1073/pnas.2009852117
- https://www.pnas.org/content/pnas/117/39/24076.full.pdf
- OA Status
- bronze
- Cited By
- 19
- References
- 51
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W3085092325Canonical identifier for this work in OpenAlex
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https://doi.org/10.1073/pnas.2009852117Digital Object Identifier
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Polyamorphism of vapor-deposited amorphous selenium in response to lightWork title
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articleOpenAlex work type
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enPrimary language
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2020Year of publication
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2020-09-15Full publication date if available
- Authors
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Aixi Zhang, Yi Jin, Tianyi Liu, R. B. Stephens, Zahra FakhraaiList of authors in order
- Landing page
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https://doi.org/10.1073/pnas.2009852117Publisher landing page
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https://www.pnas.org/content/pnas/117/39/24076.full.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://www.pnas.org/content/pnas/117/39/24076.full.pdfDirect OA link when available
- Concepts
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Polyamorphism, Selenium, Amorphous solid, Materials science, Chemical physics, Chemistry, Crystallography, MetallurgyTop concepts (fields/topics) attached by OpenAlex
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19Total citation count in OpenAlex
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2025: 4, 2024: 3, 2023: 4, 2022: 3, 2021: 4Per-year citation counts (last 5 years)
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51Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W1978005636, https://openalex.org/W2047193614, https://openalex.org/W2315966892, https://openalex.org/W2604609294, https://openalex.org/W2591283900, https://openalex.org/W1915014438, https://openalex.org/W2742747672, https://openalex.org/W2798196287, https://openalex.org/W1987005947, https://openalex.org/W2123000849, https://openalex.org/W2058873955, https://openalex.org/W2011630584, https://openalex.org/W2750985976, https://openalex.org/W2236510725, https://openalex.org/W2766760946, https://openalex.org/W2896831208, https://openalex.org/W2939290652, https://openalex.org/W2587483327, https://openalex.org/W1984312308, https://openalex.org/W3010495681, https://openalex.org/W2731507999, https://openalex.org/W2905667077, https://openalex.org/W2010409264, https://openalex.org/W1908545617, https://openalex.org/W2081228463, https://openalex.org/W1980922972, https://openalex.org/W2051677291, https://openalex.org/W2638115400, https://openalex.org/W2070868570, https://openalex.org/W2027862358, https://openalex.org/W2042770057, https://openalex.org/W2040816685, https://openalex.org/W2169014472, https://openalex.org/W2092564101, https://openalex.org/W2664016847, https://openalex.org/W2313970965, https://openalex.org/W2324374144, https://openalex.org/W2130671225, https://openalex.org/W2149530530, https://openalex.org/W1983681179, https://openalex.org/W2147080466, https://openalex.org/W2086486371, https://openalex.org/W2626213617, https://openalex.org/W2511085640, https://openalex.org/W1510599067, https://openalex.org/W2055462520, https://openalex.org/W2019083809, https://openalex.org/W2948866532, https://openalex.org/W2061353225, https://openalex.org/W2022237498, https://openalex.org/W2032564369 |
| referenced_works_count | 51 |
| abstract_inverted_index.a | 5, 38, 84 |
| abstract_inverted_index.We | 58 |
| abstract_inverted_index.at | 79 |
| abstract_inverted_index.be | 89 |
| abstract_inverted_index.is | 83 |
| abstract_inverted_index.of | 45 |
| abstract_inverted_index.on | 50 |
| abstract_inverted_index.or | 108 |
| abstract_inverted_index.to | 41, 75, 91, 95 |
| abstract_inverted_index.and | 12, 26, 48, 69 |
| abstract_inverted_index.are | 102 |
| abstract_inverted_index.can | 18, 88 |
| abstract_inverted_index.due | 74 |
| abstract_inverted_index.has | 4 |
| abstract_inverted_index.not | 103 |
| abstract_inverted_index.the | 43, 80 |
| abstract_inverted_index.This | 15, 82 |
| abstract_inverted_index.a-Se | 37 |
| abstract_inverted_index.bond | 23 |
| abstract_inverted_index.less | 65 |
| abstract_inverted_index.more | 67, 71 |
| abstract_inverted_index.role | 44 |
| abstract_inverted_index.show | 59 |
| abstract_inverted_index.that | 60, 86, 101 |
| abstract_inverted_index.upon | 29 |
| abstract_inverted_index.used | 90 |
| abstract_inverted_index.with | 9, 31 |
| abstract_inverted_index.Light | 34 |
| abstract_inverted_index.glass | 52 |
| abstract_inverted_index.light | 87 |
| abstract_inverted_index.makes | 36 |
| abstract_inverted_index.solid | 99 |
| abstract_inverted_index.study | 42 |
| abstract_inverted_index.vapor | 56 |
| abstract_inverted_index.(a-Se) | 3 |
| abstract_inverted_index.aging. | 109 |
| abstract_inverted_index.better | 76 |
| abstract_inverted_index.bonds. | 14 |
| abstract_inverted_index.defect | 27 |
| abstract_inverted_index.dense, | 66 |
| abstract_inverted_index.during | 54, 62 |
| abstract_inverted_index.light. | 33 |
| abstract_inverted_index.liquid | 106 |
| abstract_inverted_index.stable | 51, 72 |
| abstract_inverted_index.states | 100 |
| abstract_inverted_index.system | 40 |
| abstract_inverted_index.unique | 39 |
| abstract_inverted_index.changes | 21 |
| abstract_inverted_index.defects | 11 |
| abstract_inverted_index.network | 77 |
| abstract_inverted_index.surface | 46, 93 |
| abstract_inverted_index.through | 105 |
| abstract_inverted_index.undergo | 19 |
| abstract_inverted_index.dangling | 13 |
| abstract_inverted_index.distinct | 97 |
| abstract_inverted_index.dynamics | 49 |
| abstract_inverted_index.generate | 96 |
| abstract_inverted_index.glasses, | 73 |
| abstract_inverted_index.physical | 55 |
| abstract_inverted_index.produces | 64 |
| abstract_inverted_index.selenium | 2 |
| abstract_inverted_index.surface. | 81 |
| abstract_inverted_index.Amorphous | 1 |
| abstract_inverted_index.breakage, | 24 |
| abstract_inverted_index.formation | 28, 53, 78 |
| abstract_inverted_index.including | 22 |
| abstract_inverted_index.molecular | 7 |
| abstract_inverted_index.quenching | 107 |
| abstract_inverted_index.structure | 8, 17, 47 |
| abstract_inverted_index.accessible | 104 |
| abstract_inverted_index.deposition | 63 |
| abstract_inverted_index.manipulate | 92 |
| abstract_inverted_index.properties | 94 |
| abstract_inverted_index.complicated | 6 |
| abstract_inverted_index.deposition. | 57 |
| abstract_inverted_index.kinetically | 70 |
| abstract_inverted_index.sensitivity | 35 |
| abstract_inverted_index.significant | 20 |
| abstract_inverted_index.Significance | 0 |
| abstract_inverted_index.anisotropic, | 68 |
| abstract_inverted_index.illumination | 30, 61 |
| abstract_inverted_index.polyamorphic | 98 |
| abstract_inverted_index.above-bandgap | 32 |
| abstract_inverted_index.demonstration | 85 |
| abstract_inverted_index.reconnection, | 25 |
| abstract_inverted_index.light-sensitive | 16 |
| abstract_inverted_index.overcoordinated | 10 |
| cited_by_percentile_year.max | 98 |
| cited_by_percentile_year.min | 89 |
| corresponding_author_ids | https://openalex.org/A5088670364 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 5 |
| corresponding_institution_ids | https://openalex.org/I79576946 |
| citation_normalized_percentile.value | 0.72824252 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |